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@ARTICLE{Schwartzkopf:455138,
      author       = {Schwartzkopf, Matthias and Wöhnert, Sven-Jannik and
                      Waclawek, Vivian and Carstens, Niko and Rothkirch, André
                      and Rubeck, Jan and Gensch, Marc and Drewes, Jonas and
                      Polonskyi, Oleksandr and Strunskus, Thomas and Hinz,
                      Alexander M. and Schaper, Simon J. and Körstgens, Volker
                      and Müller-Buschbaum, Peter and Faupel, Franz and Roth,
                      Stephan V.},
      title        = {{R}eal-time insight into nanostructure evolution during the
                      rapid formation of ultra-thin gold layers on polymers},
      journal      = {Nanoscale horizons},
      volume       = {6},
      number       = {2},
      issn         = {2055-6764},
      address      = {Cambridge},
      publisher    = {Royal Society of Chemistry},
      reportid     = {PUBDB-2021-00953},
      pages        = {132 - 138},
      year         = {2021},
      note         = {Waiting for fulltext},
      abstract     = {Ultra-thin metal layers on polymer thin films attract
                      tremendous research interest for advanced flexible
                      optoelectronic applications, including organic
                      photovoltaics, light emitting diodes and sensors. To realize
                      the large-scale production of such metal–polymer hybrid
                      materials, high rate sputter deposition is of particular
                      interest. Here, we witness the birth of a metal–polymer
                      hybrid material by quantifying in situ with unprecedented
                      time-resolution of 0.5 ms the temporal evolution of
                      interfacial morphology during the rapid formation of
                      ultra-thin gold layers on thin polystyrene films. We monitor
                      average non-equilibrium cluster geometries, transient
                      interface morphologies and the effective near-surface gold
                      diffusion. At 1 s sputter deposition, the polymer matrix has
                      already been enriched with $1\%$ gold and an intermixing
                      layer has formed with a depth of over 3.5 nm. Furthermore,
                      we experimentally observe unexpected changes in aspect
                      ratios of ultra-small gold clusters growing in the vicinity
                      of polymer chains. For the first time, this approach enables
                      four-dimensional insights at atomic scales during the gold
                      growth under non-equilibrium conditions.},
      cin          = {FS-PET-D / DOOR ; HAS-User / FS-EC},
      ddc          = {540},
      cid          = {I:(DE-H253)FS-PET-D-20190712 / I:(DE-H253)HAS-User-20120731
                      / I:(DE-H253)FS-EC-20120731},
      pnm          = {632 - Materials – Quantum, Complex and Functional
                      Materials (POF4-632) / 6G3 - PETRA III (DESY) (POF4-6G3) /
                      RO4638/1-1 - In-situ Untersuchungen zu Kondensation,
                      Nukleation und Wachstum von Metallfilmen und Nanostrukturen
                      auf organischen Oberflächen während Sputterbeschichtung
                      (238058777)},
      pid          = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G3 /
                      G:(GEPRIS)238058777},
      experiment   = {EXP:(DE-H253)P-P03-20150101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:33290482},
      UT           = {WOS:000617006200004},
      doi          = {10.1039/D0NH00538J},
      url          = {https://bib-pubdb1.desy.de/record/455138},
}