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001     454942
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024 7 _ |a 10.1038/s41598-021-82518-4
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100 1 _ |a Kielgast, Fridtjof
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245 _ _ |a Revealing noncollinear magnetic ordering at the atomic scale via XMCD
260 _ _ |a [London]
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520 _ _ |a Mass-selected V and Fe monomers, as well as the heterodimer Fe1V1, were deposited on a Cu(001) surface. Their electronic and magnetic properties were investigated via X-ray absorption (XAS) and X-ray magnetic circular dichroism (XMCD) spectroscopy. Anisotropies in the magnetic moments of the deposited species could be examined by means of angle resolving XMCD, i.e. changing the X-ray angle of incidence. A weak adatom-substrate-coupling was found for both elements and, using group theoretical arguments, the ground state symmetries of the adatoms were determined. For the dimer, a switching from antiparallel to parallel orientation of the respective magnetic moments was observed. We show that this is due to the existence of a noncollinear spin-flop phase in the deposited dimers, which could be observed for the first time in such a small system. Making use of the two magnetic sublattices model, we were able to find the relative orientations for the dimer magnetic moments for different incidence angles.
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700 1 _ |a Baev, Ivan
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700 1 _ |a Beeck, Torben
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700 1 _ |a Pressacco, Federico
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700 1 _ |a Martins, Michael
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773 _ _ |a 10.1038/s41598-021-82518-4
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