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@ARTICLE{Chattopadhyay:454440,
author = {Chattopadhyay, Basab and Balédent, V. and Panda, S. K. and
Yamamoto, Sh. and Duc, F. and Herrmannsdörfer, T. and
Uhlarz, M. and Gottschall, T. and Mathon, O. and Wang, Z.
and Strohm, Cornelius and Greenblatt, M. and
Foury-Leylekian, P. and Wosnitza, J.},
title = {$4f$ spin driven ferroelectric-ferromagnetic
multiferroicity in {P}r{M}n$_2${O}$_ 5$ under a magnetic
field},
journal = {Physical review / B},
volume = {102},
number = {9},
issn = {2469-9950},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {PUBDB-2021-00514},
pages = {094408},
year = {2020},
abstract = {In contrast to all other members of the $RMn_2O_5$ family
with nonzero $4f$ electrons (R = Nd to Lu), $PrMn_2O_5$ does
not show any spin driven ferroelectricity in the
magnetically ordered phase. By means of high-field electric
polarization measurements up to 45 T, we have found that
this exceptional candidate undergoes a spin driven
multiferroic phase under magnetic field. X-ray magnetic
circular dichroism studies up to 30 T at the Pr $L_2$ edge
show that this ferroelectricity originates from and directly
couples to the ferromagnetic component of the $Pr^{3+}$
spins. Experimental observations along with our generalized
gradient-approximation $+U$ calculations reveal that this
exotic ferroelectric-ferromagnetic combination stabilizes
through the exchange-striction mechanism solely driven by a
$3d−4f$-type coupling, as opposed to the other $RMn_2O_5$
members with $3d−3d$ driven
ferroelectric-antiferromagnetic-type conventional type-II
multiferroicity.},
cin = {FS-PS},
ddc = {530},
cid = {I:(DE-H253)FS-PS-20131107},
pnm = {6212 - Quantum Condensed Matter: Magnetism,
Superconductivity (POF3-621)},
pid = {G:(DE-HGF)POF3-6212},
experiment = {EXP:(DE-MLZ)External-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000566885200004},
doi = {10.1103/PhysRevB.102.094408},
url = {https://bib-pubdb1.desy.de/record/454440},
}