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| 001 | 454010 | ||
| 005 | 20250716152021.0 | ||
| 024 | 7 | _ | |a 10.1039/D0TA09671G |2 doi |
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| 100 | 1 | _ | |a Jiang, Xinyu |0 P:(DE-H253)PIP1084667 |b 0 |
| 245 | _ | _ | |a Internal nanoscale architecture and charge carrier dynamics of wide bandgap non-fullerene bulk heterojunction active layers in organic solar cells |
| 260 | _ | _ | |a London [u.a.] |c 2020 |b RSC |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Bulk heterojunction (BHJ) organic solar cells have gained increasing attention in the past few years. In this work, active layers of a wide-bandgap polymer donor with benzodithiophene units PBDB-T-2F and a non-fullerene small molecule acceptor IT-M are assembled into photovoltaic devices with different amounts of solvent additive 1,8-diiodooctane (DIO). The influence of DIO on the nanoscale film morphology and crystalline structure as well as the charge carrier dynamics of the active layers are investigated by combining grazing-incidence small-angle X-ray scattering (GISAXS), grazing-incidence wide-angle X-ray scattering (GIWAXS), X-ray reflectivity (XRR), UV-visible (UV-vis) absorption spectroscopy, X-ray photoelectron spectroscopy (XPS), time-resolved photoluminescence (TRPL) and space charge limited current measurements, which are correlated with the corresponding performance of the solar cells. At 0.5 vol% DIO addition, the wide-bandgap non-fullerene organic solar cells show the best performance due to high open-circuit voltage and short-circuit current resulting from an improved charge carrier management due to the optimal inner nanoscale morphology of the active layers in terms of surface enrichment, crystallinity and crystalline orientation. |
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| 700 | 1 | _ | |a Kim, Hongwon |b 1 |
| 700 | 1 | _ | |a Deimel, Peter S. |b 2 |
| 700 | 1 | _ | |a Chen, Wei |0 P:(DE-H253)PIP1080983 |b 3 |
| 700 | 1 | _ | |a Cao, Wei |b 4 |
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| 700 | 1 | _ | |a Schaffrinna, Roy |0 P:(DE-H253)PIP1087343 |b 7 |
| 700 | 1 | _ | |a Allegretti, Francesco |b 8 |
| 700 | 1 | _ | |a Barth, Johannes V. |b 9 |
| 700 | 1 | _ | |a Schwager, Martina |b 10 |
| 700 | 1 | _ | |a Tang, Haodong |0 0000-0002-5632-5096 |b 11 |
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| 700 | 1 | _ | |a Müller-Buschbaum, Peter |0 P:(DE-H253)PIP1007825 |b 15 |e Corresponding author |
| 773 | _ | _ | |a 10.1039/D0TA09671G |g Vol. 8, no. 44, p. 23628 - 23636 |0 PERI:(DE-600)2702232-8 |n 44 |p 23628 - 23636 |t Journal of materials chemistry / A |v 8 |y 2020 |x 2050-7496 |
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