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@ARTICLE{Tcakaev:453867,
author = {Tcakaev, A. and Zabolotnyy, V. B. and Fornari, C. I. and
Rüßmann, P. and Peixoto, T. R. F. and Stier, Fabian and
Dettbarn, M. and Kagerer, Philipp and Weschke, E. and
Schierle, E. and Bencok, P. and Rappl, P. H. O. and Abramof,
E. and Bentmann, H. and Goering, E. and Reinert, F. and
Hinkov, V.},
title = {{I}ncipient antiferromagnetism in the {E}u-doped
topological insulator {B}i$_2${T}e$_3$},
journal = {Physical review / B},
volume = {102},
number = {18},
issn = {2469-9950},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {PUBDB-2021-00231},
pages = {184401},
year = {2020},
abstract = {Rare-earth ions typically exhibit larger magnetic moments
than transition-metal ions and thus promise the opening of a
wider exchange gap in the Dirac surface states of
topological insulators. Yet in a recent photoemission study
of Eu-doped Bi$_2$Te$_3$ films, the spectra remained gapless
down to T=20 K. Here we scrutinize whether the conditions
for a substantial gap formation in this system are present
by combining spectroscopic and bulk characterization methods
with theoretical calculations. For all studied Eu doping
concentrations, our atomic multiplet analysis of the
M$_{4,5}$ x-ray absorption and magnetic circular dichroism
spectra reveals a Eu$^{2+}$ valence and confirms a large
magnetic moment, consistent with a 4$f^7$$^8S$$_{7/2}$
ground state. At temperatures below 10 K, bulk magnetometry
indicates the onset of antiferromagnetic (AFM) ordering.
This is in good agreement with density functional theory,
which predicts AFM interactions between the Eu impurities.
Our results support the notion that antiferromagnetism can
coexist with topological surface states in rare-earth-doped
Bi$_2$Te$_3$ and call for spectroscopic studies in the
Kelvin range to look for novel quantum phenomena such as the
quantum anomalous Hall effect.},
cin = {DOOR ; HAS-User},
ddc = {530},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {6G3 - PETRA III (POF3-622) / FS-Proposal: I-20181060
(I-20181060) / DFG project 390534769 - EXC 2004: Materie und
Licht für Quanteninformation (ML4Q) (390534769) / DFG
project 390858490 - EXC 2147: Komplexität und Topologie in
Quantenmaterialien (CT.QMAT) (390858490)},
pid = {G:(DE-HGF)POF3-6G3 / G:(DE-H253)I-20181060 /
G:(GEPRIS)390534769 / G:(GEPRIS)390858490},
experiment = {EXP:(DE-H253)P-P04-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000583633100005},
doi = {10.1103/PhysRevB.102.184401},
url = {https://bib-pubdb1.desy.de/record/453867},
}