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@ARTICLE{Chatterjee:453843,
author = {Chatterjee, Sayanti and Makai, Szabolcs and Morandi, Bill},
title = {{H}ydroxylamine‐{D}erived {R}eagent as a {D}ual {O}xidant
and {A}mino {G}roup {D}onor for the {I}ron‐{C}atalyzed
{P}reparation of {U}nprotected {S}ulfinamides from {T}hiols},
journal = {Angewandte Chemie / International edition},
volume = {60},
number = {2},
issn = {1521-3773},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {PUBDB-2021-00207},
pages = {758 - 765},
year = {2021},
abstract = {An iron catalyzed reaction for the selective transformation
of thiols (‐SH) to sulfinamides (‐SONH$_2$) by a direct
transfer of ‐O and free ‐NH$_2$ groups has been
developed. The reaction operates under mild conditions using
a bench stable hydroxylamine derived reagent, exhibits broad
functional group tolerance, is scalable and proceeds without
the use of any precious metal catalyst or additional
oxidant. This novel, practical reaction leads to the
formation of two distinct new bonds (S=O and S−N) in a
single step to chemoselectively form valuable, unprotected
sulfinamide products. Preliminary mechanistic studies
implicate the role of the alcoholic solvent as an oxygen
atom donor.},
cin = {DOOR ; HAS-User},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {6G3 - PETRA III (DESY) (POF4-6G3)},
pid = {G:(DE-HGF)POF4-6G3},
experiment = {EXP:(DE-H253)P-P11-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:32955152},
UT = {WOS:000587752700001},
doi = {10.1002/anie.202011138},
url = {https://bib-pubdb1.desy.de/record/453843},
}