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| 001 | 452657 | ||
| 005 | 20250716151605.0 | ||
| 024 | 7 | _ | |a 10.1126/science.abb9385 |2 doi |
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| 100 | 1 | _ | |a Kim, Kyung Hwan |b 0 |
| 245 | _ | _ | |a Experimental observation of the liquid-liquid transition in bulk supercooled water under pressure |
| 260 | _ | _ | |a Washington, DC |c 2020 |b Assoc. |
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| 500 | _ | _ | |a Copyright © 2020 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. |
| 520 | _ | _ | |a We prepared bulk samples of supercooled liquid water under pressure by isochoric heating of high-density amorphous ice to temperatures of 205 ± 10 kelvin, using an infrared femtosecond laser. Because the sample density is preserved during the ultrafast heating, we could estimate an initial internal pressure of 2.5 to 3.5 kilobar in the high-density liquid phase. After heating, the sample expanded rapidly, and we captured the resulting decompression process with femtosecond x-ray laser pulses at different pump-probe delay times. A discontinuous structural change occurred in which low-density liquid domains appeared and grew on time scales between 20 nanoseconds to 3 microseconds, whereas crystallization occurs on time scales of 3 to 50 microseconds. The dynamics of the two processes being separated by more than one order of magnitude provides support for a liquid-liquid transition in bulk supercooled water. |
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| 700 | 1 | _ | |a Amann-Winkel, Katrin |b 1 |
| 700 | 1 | _ | |a Giovambattista, Nicolas |0 0000-0003-1149-0693 |b 2 |
| 700 | 1 | _ | |a Späh, Alexander |b 3 |
| 700 | 1 | _ | |a Perakis, Fivos |0 0000-0001-9863-9811 |b 4 |
| 700 | 1 | _ | |a Pathak, Harshad |b 5 |
| 700 | 1 | _ | |a Parada, Marjorie Ladd |0 0000-0003-1355-649X |b 6 |
| 700 | 1 | _ | |a Yang, Cheolhee |b 7 |
| 700 | 1 | _ | |a Mariedahl, Daniel |b 8 |
| 700 | 1 | _ | |a Eklund, Tobias |0 0000-0002-5851-3939 |b 9 |
| 700 | 1 | _ | |a Lane, Thomas. J. |0 0000-0003-2627-4432 |b 10 |
| 700 | 1 | _ | |a You, Seonju |b 11 |
| 700 | 1 | _ | |a Jeong, Sangmin |0 0000-0003-0694-6721 |b 12 |
| 700 | 1 | _ | |a Weston, Matthew |b 13 |
| 700 | 1 | _ | |a Lee, Jae Hyuk |b 14 |
| 700 | 1 | _ | |a Eom, Intae |0 0000-0002-3390-4052 |b 15 |
| 700 | 1 | _ | |a Kim, Minseok |0 0000-0002-2504-1314 |b 16 |
| 700 | 1 | _ | |a Park, Jaeku |b 17 |
| 700 | 1 | _ | |a Chun, Sae Hwan |b 18 |
| 700 | 1 | _ | |a Poole, Peter H. |0 0000-0001-5985-0585 |b 19 |
| 700 | 1 | _ | |a Nilsson, Anders |0 0000-0003-1968-8696 |b 20 |e Corresponding author |
| 773 | _ | _ | |a 10.1126/science.abb9385 |g Vol. 370, no. 6519, p. 978 - 982 |0 PERI:(DE-600)2089761-3 |n 6519 |p 978 - 982 |t Science / Science now |v 370 |y 2020 |x 1095-9203 |
| 856 | 4 | _ | |y OpenAccess |u https://bib-pubdb1.desy.de/record/452657/files/Experimental%20obersvation%20of%20the%20liquid-liquid%20transition%20in%20bulk%20supercooled%20water%20under%20pressure-1.pdf |
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