000452657 001__ 452657
000452657 005__ 20250716151605.0
000452657 0247_ $$2doi$$a10.1126/science.abb9385
000452657 0247_ $$2ISSN$$a0036-8075
000452657 0247_ $$2ISSN$$a1095-9203
000452657 0247_ $$2ISSN$$a1947-8062
000452657 0247_ $$2altmetric$$aaltmetric:94611194
000452657 0247_ $$2pmid$$apmid:33214280
000452657 0247_ $$2WOS$$aWOS:000594441500051
000452657 0247_ $$2datacite_doi$$a10.3204/PUBDB-2020-04811
000452657 0247_ $$2openalex$$aopenalex:W3102571085
000452657 037__ $$aPUBDB-2020-04811
000452657 041__ $$aEnglish
000452657 082__ $$a320
000452657 1001_ $$aKim, Kyung Hwan$$b0
000452657 245__ $$aExperimental observation of the liquid-liquid transition in bulk supercooled water under pressure
000452657 260__ $$aWashington, DC$$bAssoc.$$c2020
000452657 3367_ $$2DRIVER$$aarticle
000452657 3367_ $$2DataCite$$aOutput Types/Journal article
000452657 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1630487810_13886
000452657 3367_ $$2BibTeX$$aARTICLE
000452657 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000452657 3367_ $$00$$2EndNote$$aJournal Article
000452657 500__ $$aCopyright © 2020 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. 
000452657 520__ $$aWe prepared bulk samples of supercooled liquid water under pressure by isochoric heating of high-density amorphous ice to temperatures of 205 ± 10 kelvin, using an infrared femtosecond laser. Because the sample density is preserved during the ultrafast heating, we could estimate an initial internal pressure of 2.5 to 3.5 kilobar in the high-density liquid phase. After heating, the sample expanded rapidly, and we captured the resulting decompression process with femtosecond x-ray laser pulses at different pump-probe delay times. A discontinuous structural change occurred in which low-density liquid domains appeared and grew on time scales between 20 nanoseconds to 3 microseconds, whereas crystallization occurs on time scales of 3 to 50 microseconds. The dynamics of the two processes being separated by more than one order of magnitude provides support for a liquid-liquid transition in bulk supercooled water.
000452657 536__ $$0G:(DE-HGF)POF3-6215$$a6215 - Soft Matter, Health and Life Sciences (POF3-621)$$cPOF3-621$$fPOF III$$x0
000452657 588__ $$aDataset connected to CrossRef
000452657 693__ $$0EXP:(DE-MLZ)External-20140101$$5EXP:(DE-MLZ)External-20140101$$eMeasurement at external facility$$x0
000452657 7001_ $$aAmann-Winkel, Katrin$$b1
000452657 7001_ $$00000-0003-1149-0693$$aGiovambattista, Nicolas$$b2
000452657 7001_ $$aSpäh, Alexander$$b3
000452657 7001_ $$00000-0001-9863-9811$$aPerakis, Fivos$$b4
000452657 7001_ $$aPathak, Harshad$$b5
000452657 7001_ $$00000-0003-1355-649X$$aParada, Marjorie Ladd$$b6
000452657 7001_ $$aYang, Cheolhee$$b7
000452657 7001_ $$aMariedahl, Daniel$$b8
000452657 7001_ $$00000-0002-5851-3939$$aEklund, Tobias$$b9
000452657 7001_ $$00000-0003-2627-4432$$aLane, Thomas. J.$$b10
000452657 7001_ $$aYou, Seonju$$b11
000452657 7001_ $$00000-0003-0694-6721$$aJeong, Sangmin$$b12
000452657 7001_ $$aWeston, Matthew$$b13
000452657 7001_ $$aLee, Jae Hyuk$$b14
000452657 7001_ $$00000-0002-3390-4052$$aEom, Intae$$b15
000452657 7001_ $$00000-0002-2504-1314$$aKim, Minseok$$b16
000452657 7001_ $$aPark, Jaeku$$b17
000452657 7001_ $$aChun, Sae Hwan$$b18
000452657 7001_ $$00000-0001-5985-0585$$aPoole, Peter H.$$b19
000452657 7001_ $$00000-0003-1968-8696$$aNilsson, Anders$$b20$$eCorresponding author
000452657 773__ $$0PERI:(DE-600)2089761-3$$a10.1126/science.abb9385$$gVol. 370, no. 6519, p. 978 - 982$$n6519$$p978 - 982$$tScience / Science now$$v370$$x1095-9203$$y2020
000452657 8564_ $$uhttps://bib-pubdb1.desy.de/record/452657/files/Experimental%20obersvation%20of%20the%20liquid-liquid%20transition%20in%20bulk%20supercooled%20water%20under%20pressure-1.pdf$$yOpenAccess
000452657 8564_ $$uhttps://bib-pubdb1.desy.de/record/452657/files/Experimental%20obersvation%20of%20the%20liquid-liquid%20transition%20in%20bulk%20supercooled%20water%20under%20pressure-1.pdf?subformat=pdfa$$xpdfa$$yOpenAccess
000452657 909CO $$ooai:bib-pubdb1.desy.de:452657$$pdnbdelivery$$pdriver$$pVDB$$popen_access$$popenaire
000452657 9101_ $$0I:(DE-588b)2008985-5$$60000-0003-2627-4432$$aDeutsches Elektronen-Synchrotron$$b10$$kDESY
000452657 9101_ $$0I:(DE-H253)_CFEL-20120731$$60000-0003-2627-4432$$aCentre for Free-Electron Laser Science$$b10$$kCFEL
000452657 9131_ $$0G:(DE-HGF)POF3-621$$1G:(DE-HGF)POF3-620$$2G:(DE-HGF)POF3-600$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$9G:(DE-HGF)POF3-6215$$aDE-HGF$$bForschungsbereich Materie$$lVon Materie zu Materialien und Leben$$vIn-house research on the structure, dynamics and function of matter$$x0
000452657 9132_ $$0G:(DE-HGF)POF4-633$$1G:(DE-HGF)POF4-630$$2G:(DE-HGF)POF4-600$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$aDE-HGF$$bForschungsbereich Materie$$lMatter and Technologies$$vLife Sciences – Building Blocks of Life: Structure and Function$$x0
000452657 9141_ $$y2020
000452657 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)1050$$2StatID$$aDBCoverage$$bBIOSIS Previews$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)1190$$2StatID$$aDBCoverage$$bBiological Abstracts$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)0600$$2StatID$$aDBCoverage$$bEbsco Academic Search$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)1040$$2StatID$$aDBCoverage$$bZoological Record$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)1200$$2StatID$$aDBCoverage$$bChemical Reactions$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)1060$$2StatID$$aDBCoverage$$bCurrent Contents - Agriculture, Biology and Environmental Sciences$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)1030$$2StatID$$aDBCoverage$$bCurrent Contents - Life Sciences$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)1210$$2StatID$$aDBCoverage$$bIndex Chemicus$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)0113$$2StatID$$aWoS$$bScience Citation Index Expanded$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
000452657 915__ $$0StatID:(DE-HGF)0030$$2StatID$$aPeer Review$$bASC$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bSCIENCE : 2018$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)0160$$2StatID$$aDBCoverage$$bEssential Science Indicators$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)9940$$2StatID$$aIF >= 40$$bSCIENCE : 2018$$d2020-09-15
000452657 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List$$d2020-09-15
000452657 9201_ $$0I:(DE-H253)FS-CFEL-1-20120731$$kFS-CFEL-1$$lCFEL-Coherent X-Ray Imaging$$x0
000452657 9201_ $$0I:(DE-H253)CFEL-I-20161114$$kCFEL-I$$lFS-CFEL-1 (Group Leader: Henry Chapman)$$x1
000452657 980__ $$ajournal
000452657 980__ $$aVDB
000452657 980__ $$aUNRESTRICTED
000452657 980__ $$aI:(DE-H253)FS-CFEL-1-20120731
000452657 980__ $$aI:(DE-H253)CFEL-I-20161114
000452657 9801_ $$aFullTexts