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@ARTICLE{Li:452549,
author = {Li, Weixing and Quesada Moreno, Maria del Mar and Pinacho
Morante, Pablo and Schnell, Melanie},
title = {{U}nlocking the {W}ater {T}rimer {L}oop: {I}sotpic {S}tudy
of {B}enzophenone-$({H}_{2}{O})_{1-3}$ {C}lusters with
{R}otational {S}pectroscopy},
journal = {Angewandte Chemie / International edition},
volume = {60},
number = {10},
issn = {0570-0833},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {PUBDB-2020-04749},
pages = {5323 – 5330},
year = {2021},
abstract = {Examined here are the structures of complexes of
benzophenone microsolvated with up to three water molecules
by using broadband rotational spectroscopy and the cold
conditions of a molecular jet. The analysis shows that the
water molecules dock sideways on benzophenone for the water
monomer and dimer moieties, and they move above one of the
aromatic rings when the water cluster grows to the trimer.
The rotational spectra shows that the water trimer moiety in
the complex adopts an open-loop arrangement .Ab initio
calculations face a dilemma of identifying the global
minimum between the open loop and the closed loop, which is
only solved when zero-point vibrational energy correction is
applied. An OH···p bond and a Bürgi-Dunitz interaction
between benzophenone and the water trimer are present in the
cluster. This work shows the subtle balance between
water–water and water–solute interactions when the
solute molecule offers several different anchor sites for
water molecules.},
cin = {FS-SMP},
ddc = {540},
cid = {I:(DE-H253)FS-SMP-20171124},
pnm = {631 - Matter – Dynamics, Mechanisms and Control
(POF4-631) / DFG project 271359857 - Intra- und
untermolekulare Dispersionskräfte: Beiträge zum
Verständnis von Komplexbildung, Aggregation und dem Effekt
der Solvatisierung mit Hilfe eines bottom-up Ansatzes
(271359857)},
pid = {G:(DE-HGF)POF4-631 / G:(GEPRIS)271359857},
experiment = {EXP:(DE-MLZ)NOSPEC-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:33289239},
UT = {WOS:000611117100001},
doi = {10.1002/anie.202013899},
url = {https://bib-pubdb1.desy.de/record/452549},
}