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@ARTICLE{Josts:442859,
author = {Josts, Inokentijs and Gao, Yunyun and Monteiro, Diana C. F.
and Niebling, Stephan and Nitsche, Julius and Veith,
Katharina and Gräwert, Tobias W. and Blanchet, Clement E.
and Schroer, Martin A. and Huse, Nils and Pearson, Arwen R.
and Svergun, Dmitri I. and Tidow, Henning},
title = {{S}tructural {K}inetics of {M}sb{A} {I}nvestigated by
{S}topped-{F}low {T}ime-{R}esolved {S}mall-{A}ngle {X}-{R}ay
{S}cattering},
journal = {Structure},
volume = {28},
number = {3},
issn = {0969-2126},
address = {Cambridge, Mass.},
publisher = {Cell Press},
reportid = {PUBDB-2020-03264},
pages = {348 - 354},
year = {2020},
abstract = {Recent structures of full-length ATP-binding cassette (ABC)
transporter MsbA in different states indicate large
conformational changes during the reaction cycle that
involve transient dimerization of its nucleotide-binding
domains (NBDs). However, a detailed molecular understanding
of the structural changes and associated kinetics of MsbA
upon ATP binding and hydrolysis is still missing. Here, we
employed time-resolved small-angle X-ray scattering,
initiated by stopped-flow mixing, to investigate the
kinetics and accompanying structural changes of NBD
dimerization (upon ATP binding) and subsequent dissociation
(upon ATP hydrolysis) in the context of isolated NBDs as
well as full-length MsbA in lipid nanodiscs. Our data
allowed us to structurally characterize the major states
involved in the process and determine time constants for NBD
dimerization and dissociation. In the full-length protein,
these structural transitions occur on much faster time
scales, indicating close-proximity effects and structural
coupling of the transmembrane domains with the NBDs.},
cin = {EMBL-User / CSSB-EMBL / EMBL},
ddc = {540},
cid = {I:(DE-H253)EMBL-User-20120814 /
I:(DE-H253)CSSB-EMBL-20141216 / I:(DE-H253)EMBL-20120731},
pnm = {6G3 - PETRA III (POF3-622) / DFG project 390715994 - EXC
2056: CUI: Advanced Imaging of Matter (390715994) / DFG
project 194651731 - EXC 1074: Hamburger Zentrum für
ultraschnelle Beobachtung (CUI): Struktur, Dynamik und
Kontrolle von Materie auf atomarer Skala (194651731)},
pid = {G:(DE-HGF)POF3-6G3 / G:(GEPRIS)390715994 /
G:(GEPRIS)194651731},
experiment = {EXP:(DE-H253)P-P12-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:31899087},
UT = {WOS:000518466100010},
doi = {10.1016/j.str.2019.12.001},
url = {https://bib-pubdb1.desy.de/record/442859},
}