TY - JOUR
AU - Dziarzhytski, Siarhei
AU - Biednov, M.
AU - Dicke, B.
AU - Wang, A.
AU - Miedema, P. S.
AU - Engel, R. Y.
AU - Schunck, Jan
AU - Redlin, H.
AU - Weigelt, Holger
AU - Siewert, F.
AU - Behrens, Christopher
AU - Sinha, M.
AU - Schulte, Amelie
AU - Grimm-Lebsanft, B.
AU - Chiuzbăian, S. G.
AU - Wurth, W.
AU - Beye, M.
AU - Rübhausen, M.
AU - Brenner, Guenter
TI - The TRIXS end-station for femtosecond time-resolved resonant inelastic X-ray free-electron laser FLASH
JO - Structural dynamics
VL - 7
IS - 5
SN - 2329-7778
CY - Melville, NY
PB - AIP Publishing LLC
M1 - PUBDB-2020-03171
SP - 054301 (1-12)
PY - 2020
AB - We present the experimental end-station TRIXS dedicated to time-resolved soft x-ray resonant inelastic x-ray scattering (RIXS) experiments on solid samples at the free-electron laser FLASH. Using monochromatized ultrashort femtosecond XUV/soft x-ray photon pulses in combination with a synchronized optical laser in a pump-probe scheme, the TRIXS setup allows measuring sub-picosecond time-resolved high-resolution RIXS spectra in the energy range from 35 eV to 210 eV, thus spanning the M-edge (M<sub>1</sub> and M<sub>2,3</sub>) absorption resonances of 3d transition metals and N<sub>4,5</sub>-edges of rare earth elements. A Kirkpatrick–Baez refocusing mirror system at the first branch of the plane grating monochromator beamline (PG1) provides a focus of (6 × 6) μm<sup>2</sup> (FWHM) at the sample. The RIXS spectrometer reaches an energy resolution of 35–160 meV over the entire spectral range. The optical laser system based on a chirped pulse optical parametric amplifier provides approximately 100 fs (FWHM) long photon pulses at the fundamental wavelength of 800 nm and a fluence of 120 mJ/cm<sup>2</sup> at a sample for optical pump-XUV probe measurements. Furthermore, optical frequency conversion enables experiments at 400 nm or 267 nm with a fluence of 80 and 30 mJ/cm<sup>2</sup>, respectively. Some of the first (pump-probe) RIXS spectra measured with this setup are shown. The measured time resolution for time-resolved RIXS measurements has been characterized as 287 fs (FWHM) for the used energy resolution.
LB - PUB:(DE-HGF)16
C6 - pmid:32953941
UR - <Go to ISI:>//WOS:000569934600001
DO - DOI:10.1063/4.0000029
UR - https://bib-pubdb1.desy.de/record/442673
ER -