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000429371 0247_ $$2doi$$a10.1016/j.jnoncrysol.2019.119533
000429371 0247_ $$2ISSN$$a0022-3093
000429371 0247_ $$2ISSN$$a1873-4812
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000429371 041__ $$aEnglish
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000429371 1001_ $$0P:(DE-HGF)0$$aStronski, A.$$b0
000429371 245__ $$aStoichiometric deviations in bond distances in the mixed $As_{2}S_{3}-As_{2}Se_{3}$ system: Raman spectroscopy and EXAFS studies
000429371 260__ $$aAmsterdam [u.a.]$$bElsevier Science$$c2019
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000429371 500__ $$a© Elsevier B.V.; Full published version in progress; Post referee fulltext in progress; Embargo 12 months from publication
000429371 520__ $$aRaman spectroscopy and extended X-ray absorption fine structure (EXAFS) spectroscopy have been applied to find evidence for isostructural substitution of chalcogen atoms in pyramidal structural units of network glasses from stoichiometric/pseudo-binary As2S3-As2Se3 system. The obtained values of the nearest neighbours atomic distance (rAs-Se = 2.37 ± 0.01 Å; rAs-S = 2.33 ± 0.01 Å for As40Se30S30) suggest the existence of mixed AsS2Se and AsSe2S pyramids in which each of As atoms is bonded with S and/or Se atoms in relation to S/Se ratio in composition, while Se atoms are bonded only with As ones with the same bond distance in the form of = As-Se-As = bridges that connect the main pyramidal structural units. No evidence for existence of heteroatomic or heteronuclear SeS bonding is found for the examined glasses
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000429371 7001_ $$0P:(DE-H253)PIP1008282$$aKavetskyy, T.$$b1
000429371 7001_ $$0P:(DE-HGF)0$$aRevutska, L.$$b2
000429371 7001_ $$0P:(DE-H253)PIP1007906$$aKaban, I.$$b3
000429371 7001_ $$0P:(DE-HGF)0$$aShportko, K.$$b4
000429371 7001_ $$0P:(DE-HGF)0$$aBaran, J.$$b5
000429371 7001_ $$0P:(DE-HGF)0$$aTrzebiatowska, M.$$b6
000429371 773__ $$0PERI:(DE-600)1500501-x$$a10.1016/j.jnoncrysol.2019.119533$$gVol. 521, p. 119533 -$$p119533 (6 pages)$$tJournal of non-crystalline solids$$v521$$x0022-3093$$y2019
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