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024 7 _ |a 10.1038/s41467-019-10657-4
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100 1 _ |a Jolly, Spencer Windhorst
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245 _ _ |a Spectral phase control of interfering chirped pulses for high-energy narrowband terahertz generation
260 _ _ |a [London]
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520 _ _ |a Highly-efficient optical generation of narrowband terahertz radiation enables unexplored technologies and sciences from compact electron acceleration to charge manipulation in solids. State-of-the-art conversion efficiencies are currently achieved using difference-frequency generation driven by temporal beating of chirped pulses but remain, however, far lower than desired or predicted. Here we show that high-order spectral phase fundamentally limits the efficiency of narrowband difference-frequency generation using chirped-pulse beating and resolve this limitation by introducing a novel technique based on tuning the relative spectral phase of the pulses. For optical terahertz generation, we demonstrate a 13-fold enhancement in conversion efficiency for 1%-bandwidth, 0.361 THz pulses, yielding a record energy of 0.6 mJ and exceeding previous optically-generated energies by over an order of magnitude. Our results prove the feasibility of millijoule-scale applications like terahertz-based electron accelerators and light sources and solve the long-standing problem of temporal irregularities in the pulse trains generated by interfering chirped pulses.
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700 1 _ |a Matlis, Nicholas H.
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700 1 _ |a Ahr, Frederike
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700 1 _ |a Leroux, Vincent
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700 1 _ |a Eichner, Timo
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700 1 _ |a Calendron, Anne-Laure
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700 1 _ |a Ishizuki, Hideki
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700 1 _ |a Taira, Takunori
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700 1 _ |a Kärtner, Franz X.
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700 1 _ |a Maier, Andreas R.
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773 _ _ |a 10.1038/s41467-019-10657-4
|g Vol. 10, no. 1, p. 2591
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856 4 _ |u https://www.nature.com/articles/s41467-019-10657-4#citeas
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