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000428283 1001_ $$0P:(DE-H253)PIP1023403$$aJolly, Spencer Windhorst$$b0$$eCorresponding author
000428283 245__ $$aSpectral phase control of interfering chirped pulses for high-energy narrowband terahertz generation
000428283 260__ $$a[London]$$bNature Publishing Group UK$$c2019
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000428283 520__ $$aHighly-efficient optical generation of narrowband terahertz radiation enables unexplored technologies and sciences from compact electron acceleration to charge manipulation in solids. State-of-the-art conversion efficiencies are currently achieved using difference-frequency generation driven by temporal beating of chirped pulses but remain, however, far lower than desired or predicted. Here we show that high-order spectral phase fundamentally limits the efficiency of narrowband difference-frequency generation using chirped-pulse beating and resolve this limitation by introducing a novel technique based on tuning the relative spectral phase of the pulses. For optical terahertz generation, we demonstrate a 13-fold enhancement in conversion efficiency for 1%-bandwidth, 0.361 THz pulses, yielding a record energy of 0.6 mJ and exceeding previous optically-generated energies by over an order of magnitude. Our results prove the feasibility of millijoule-scale applications like terahertz-based electron accelerators and light sources and solve the long-standing problem of temporal irregularities in the pulse trains generated by interfering chirped pulses.
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000428283 7001_ $$0P:(DE-H253)PIP1026174$$aMatlis, Nicholas H.$$b1
000428283 7001_ $$0P:(DE-H253)PIP1019231$$aAhr, Frederike$$b2
000428283 7001_ $$aLeroux, Vincent$$b3
000428283 7001_ $$0P:(DE-H253)PIP1024414$$aEichner, Timo$$b4
000428283 7001_ $$0P:(DE-H253)PIP1014959$$aCalendron, Anne-Laure$$b5
000428283 7001_ $$0P:(DE-HGF)0$$aIshizuki, Hideki$$b6
000428283 7001_ $$0P:(DE-HGF)0$$aTaira, Takunori$$b7
000428283 7001_ $$0P:(DE-H253)PIP1013198$$aKärtner, Franz X.$$b8
000428283 7001_ $$aMaier, Andreas R.$$b9
000428283 773__ $$0PERI:(DE-600)2553671-0$$a10.1038/s41467-019-10657-4$$gVol. 10, no. 1, p. 2591$$n1$$p2591$$tNature Communications$$v10$$x2041-1723$$y2019
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