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@ARTICLE{Yachmenev:426632,
      author       = {Yachmenev, Andrey and Onvlee, Jolijn and Zak, Emil and
                      Owens, Alec and Küpper, Jochen},
      title        = {{F}ield-induced diastereomers for chiral separation},
      journal      = {Physical review letters},
      volume       = {123},
      number       = {24},
      issn         = {0031-9007},
      address      = {College Park, Md.},
      publisher    = {APS},
      reportid     = {PUBDB-2019-03812, arXiv:1905.07166},
      pages        = {243202},
      year         = {2019},
      abstract     = {A novel approach for the state-specific enantiomeric
                      enrichment and the spatial separation ofenantiomers is
                      presented. Our scheme utilizes techniques from strong-field
                      laser physics, specificallyan optical centrifuge in
                      conjunction with a static electric field, to create a chiral
                      field with definedhandedness. Molecular enantiomers
                      experience unique rotational excitation dynamics and thiscan
                      be exploited to spatially separate the enantiomers using
                      electrostatic deflection. Notably,
                      therotational-state-specific enantiomeric enhancement and
                      its handedness is fully controllable. Toexplain these
                      effects, the conceptual framework of field-induced
                      diastereomers of a chiral molecule isintroduced and
                      computationally demonstrated through robust
                      quantum-mechanical simulations onthe prototypical chiral
                      molecule propylene oxide (C$_3$H$_6$O), for which ensembles
                      with an enantiomericexcess of up to 30 \% were obtained.},
      cin          = {FS-CFEL-CMI / FS-CFEL-1 / UNI/CUI / UNI/EXP},
      ddc          = {530},
      cid          = {I:(DE-H253)FS-CFEL-CMI-20220405 /
                      I:(DE-H253)FS-CFEL-1-20120731 /
                      $I:(DE-H253)UNI_CUI-20121230$ /
                      $I:(DE-H253)UNI_EXP-20120731$},
      pnm          = {6211 - Extreme States of Matter: From Cold Ions to Hot
                      Plasmas (POF3-621) / COMOTION - Controlling the Motion of
                      Complex Molecules and Particles (614507) / DFG project
                      281310165 - Abbildung chemischer Dynamik mittels
                      laserinduzierter Elektronenbeugung im
                      Molekülkoordinatensystem (281310165) / DFG project
                      390715994 - EXC 2056: CUI: Advanced Imaging of Matter
                      (390715994) / DFG project 194651731 - EXC 1074: Hamburger
                      Zentrum für ultraschnelle Beobachtung (CUI): Struktur,
                      Dynamik und Kontrolle von Materie auf atomarer Skala
                      (194651731) / Ex-Net-0002-Phase2-3 - Advanced Imaging of
                      Matter: Structure, Dynamics and Control on the Atomic Scale
                      - AIM $(2018_Ex-Net-0002-Phase2-3)$},
      pid          = {G:(DE-HGF)POF3-6211 / G:(EU-Grant)614507 /
                      G:(GEPRIS)281310165 / G:(GEPRIS)390715994 /
                      G:(GEPRIS)194651731 / $G:(DE-HGF)2018_Ex-Net-0002-Phase2-3$},
      experiment   = {EXP:(DE-MLZ)NOSPEC-20140101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:31922822},
      UT           = {WOS:000501809100003},
      eprint       = {1905.07166},
      howpublished = {arXiv:1905.07166},
      archivePrefix = {arXiv},
      SLACcitation = {$\%\%CITATION$ = $arXiv:1905.07166;\%\%$},
      doi          = {10.1103/PhysRevLett.123.243202},
      url          = {https://bib-pubdb1.desy.de/record/426632},
}