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@ARTICLE{Bernhard:424575,
author = {Bernhard, D. and Fatima, Mariyam and Poblotzki, A. and
Steber, A. L. and Pérez, C. and Suhm, M. A. and Schnell, M.
and Gerhards, M.},
title = {{D}ispersion-controlled docking preference:
multi-spectroscopic study on complexes of dibenzofuran with
alcohols and water},
journal = {Physical chemistry, chemical physics},
volume = {21},
number = {29},
issn = {1463-9084},
address = {Cambridge},
publisher = {RSC Publ.},
reportid = {PUBDB-2019-03006},
pages = {16032 - 16046},
year = {2019},
abstract = {The structural preferences within a series of
dibenzofuran–solvent complexes have been investigated by
electronic, vibrational, and rotational spectroscopic
methods probing supersonic jet expansions. The experimental
study is accompanied by a detailed theoretical analysis
including dispersion-corrected density functional theory,
symmetry adapted perturbation theory, as well as coupled
cluster approaches. The complementary, multi-spectroscopic
results reveal a preferred OH⋯O structure for the smallest
complex of dibenzofuran–water, whereas for the methanol
complex an OH⋯π isomer is simultaneously observed. For
the largest complex, dibenzofuran–tert-butyl alcohol, only
a π-bound structure is found. These comprehensive
investigations show that a completely inverse trend
regarding the docking preference is observed by comparing
the present results with the ones for analogous diphenyl
ether complexes. This can be rationalized on the basis of
the planarity/non-planarity and rigidity/flexibility of the
different systems, providing valuable insight into the
interplay between different non-covalent interactions. This
analysis is a further step towards a quantitative
description of very delicate energetic balances with the
overall goal of yielding reliable structural predictions for
non-covalently bound systems.},
cin = {FS-SMP},
ddc = {540},
cid = {I:(DE-H253)FS-SMP-20171124},
pnm = {6211 - Extreme States of Matter: From Cold Ions to Hot
Plasmas (POF3-621)},
pid = {G:(DE-HGF)POF3-6211},
experiment = {EXP:(DE-MLZ)NOSPEC-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:31304945},
UT = {WOS:000477705800007},
doi = {10.1039/C9CP02635E},
url = {https://bib-pubdb1.desy.de/record/424575},
}