% IMPORTANT: The following is UTF-8 encoded. This means that in the presence
% of non-ASCII characters, it will not work with BibTeX 0.99 or older.
% Instead, you should use an up-to-date BibTeX implementation like “bibtex8” or
% “biber”.
@ARTICLE{Rohlf:424560,
author = {Rohlf, Sebastian and Grunwald, Jan and Jasper-Toennies,
Torben and Johannsen, Sven and Diekmann, Florian and
Studniarek, Michał and Berndt, Richard and Tuczek, Felix
and Rossnagel, Kai and Gruber, Manuel},
title = {{I}nfluence of {S}ubstrate {E}lectronic {P}roperties on the
{I}ntegrity and {F}unctionality of an {A}dsorbed {F}e({II})
{S}pin-{C}rossover {C}ompound},
journal = {The journal of physical chemistry / C},
volume = {123},
number = {29},
issn = {1932-7447},
address = {Washington, DC},
publisher = {ACS},
reportid = {PUBDB-2019-02991},
pages = {17774 - 17780},
year = {2019},
note = {© American Chemical Society},
abstract = {The bistability of spin-crossover complexes on surfaces is
of great interest for potential applications. Using X-ray
absorption spectroscopy, we investigated the properties of
[Fe(pypyr(CF$_3$)$_2$)$_2$(phen)] (pypyr =
2-(2′-pyridyl)pyrrolide, phen = 1,10-phenanthroline), a
vacuum-evaporable Fe(II) complex, in direct contact to a set
of substrates. The electronic properties of these substrates
range from metallic to semiconducting. While dissociation is
observed on metal surfaces, efficient light-induced
switching is realized on semimetallic and semiconducting
surfaces. This indicates that the density of states of the
substrate at the Fermi level plays a role for the integrity
and functionality of the adsorbed compound. In an
intermediate case, namely, [Fe(pypyr(CF$_3$)$_2$)$_2$(phen)]
on graphene/Ni(111), functional and dissociated species are
found to coexist. This result indicates that some previous
studies may deserve to be reconsidered because the
possibility of coexisting intact and fragmented
spin-crossover complexes was neglected.},
cin = {FS-SXQM / UKiel},
ddc = {530},
cid = {I:(DE-H253)FS-SXQM-20190201 / I:(DE-H253)UKiel-20120814},
pnm = {6212 - Quantum Condensed Matter: Magnetism,
Superconductivity (POF3-621)},
pid = {G:(DE-HGF)POF3-6212},
experiment = {EXP:(DE-MLZ)NOSPEC-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000477785000016},
doi = {10.1021/acs.jpcc.9b02845},
url = {https://bib-pubdb1.desy.de/record/424560},
}