000423815 001__ 423815
000423815 005__ 20250716154052.0
000423815 0247_ $$2doi$$a10.1063/1.5091756
000423815 0247_ $$2datacite_doi$$a10.3204/PUBDB-2019-02676
000423815 0247_ $$2pmid$$apmid:31123698
000423815 0247_ $$2WOS$$aWOS:000474442500002
000423815 0247_ $$2openalex$$aopenalex:W2944204820
000423815 037__ $$aPUBDB-2019-02676
000423815 041__ $$aEnglish
000423815 082__ $$a500
000423815 1001_ $$0P:(DE-H253)PIP1030978$$aWenig, K.$$b0$$eCorresponding author
000423815 245__ $$aElectronic decay of core-excited HCl molecules probed by THz streaking
000423815 260__ $$aMelville, NY$$bAIP Publishing LLC$$c2019
000423815 3367_ $$2DRIVER$$aarticle
000423815 3367_ $$2DataCite$$aOutput Types/Journal article
000423815 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1718108846_3713163
000423815 3367_ $$2BibTeX$$aARTICLE
000423815 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000423815 3367_ $$00$$2EndNote$$aJournal Article
000423815 520__ $$aThe ultrafast electronic decay of HCl molecules in the time domain after resonant core excitation was measured. Here, a Cl-2p core electron was promoted to the antibonding σ* orbital initiating molecular dissociation, and simultaneously, the electronic excitation relaxes via an Auger decay. For HCl, both processes compete on similar ultrashort femtosecond time scales. In order to measure the lifetime of the core hole excitation, we collinearly superimposed 40 fs soft x-ray pulses with intense terahertz (THz) radiation from the free-electron laser in Hamburg (FLASH). Electrons emitted from the molecules are accelerated (streaked) by the THz electric field where the resulting momentum change depends on the field's phase at the instant of ionization. Evaluation of a time-shift between the delay-dependent streaking spectra of photo- and Auger electrons yields a decay constant of (11 ± 2) fs for LMM Auger electrons. For further validation, the method was also applied to the MNN Auger decay of krypton. Reproduction of the value already published in the literature confirms that a temporal resolution much below the duration of the exciting x-ray pulses can be reached.
000423815 536__ $$0G:(DE-HGF)POF3-6211$$a6211 - Extreme States of Matter: From Cold Ions to Hot Plasmas (POF3-621)$$cPOF3-621$$fPOF III$$x0
000423815 536__ $$0G:(GEPRIS)194651731$$aDFG project 194651731 - EXC 1074: Hamburger Zentrum für ultraschnelle Beobachtung (CUI): Struktur, Dynamik und Kontrolle von Materie auf atomarer Skala (194651731)$$c194651731$$x1
000423815 536__ $$0G:(GEPRIS)390715994$$aDFG project 390715994 - EXC 2056: CUI: Advanced Imaging of Matter (390715994)$$c390715994$$x2
000423815 588__ $$aDataset connected to CrossRef
000423815 693__ $$0EXP:(DE-H253)F-BL3-20150101$$1EXP:(DE-H253)FLASH-20150101$$6EXP:(DE-H253)F-BL3-20150101$$aFLASH$$fFLASH Beamline BL3$$x0
000423815 693__ $$0EXP:(DE-H253)F-ThzBL-20150101$$1EXP:(DE-H253)FLASH-20150101$$6EXP:(DE-H253)F-ThzBL-20150101$$aFLASH$$fFLASH THz Undulator Beamline$$x1
000423815 7001_ $$0P:(DE-H253)PIP1005161$$aWieland, Marek$$b1
000423815 7001_ $$0P:(DE-H253)PIP1023691$$aBaumann, Arne$$b2
000423815 7001_ $$0P:(DE-H253)PIP1030287$$aWalther, S.$$b3
000423815 7001_ $$0P:(DE-H253)PIP1028048$$aDimitriou, Anastasios$$b4
000423815 7001_ $$00000-0002-6051-0366$$aPrandolini, M. J.$$b5
000423815 7001_ $$0P:(DE-H253)PIP1023228$$aSchepp, Oliver$$b6
000423815 7001_ $$0P:(DE-H253)PIP1031019$$aBermúdez Macias, I.$$b7$$udesy
000423815 7001_ $$0P:(DE-H253)PIP1025172$$aSumfleth, Malte$$b8$$udesy
000423815 7001_ $$0P:(DE-H253)PIP1006748$$aStojanovic, N.$$b9$$udesy
000423815 7001_ $$0P:(DE-H253)PIP1002687$$aDüsterer, S.$$b10$$udesy
000423815 7001_ $$0P:(DE-H253)PIP1004087$$aRönsch-Schulenburg, Juliane$$b11$$udesy
000423815 7001_ $$0P:(DE-H253)PIP1023118$$aZapolnova, E.$$b12$$udesy
000423815 7001_ $$0P:(DE-H253)PIP1031146$$aPan, R.$$b13$$udesy
000423815 7001_ $$0P:(DE-H253)PIP1003945$$aDrescher, M.$$b14
000423815 7001_ $$0P:(DE-H253)PIP1005343$$aFruehling, Ulrike$$b15
000423815 773__ $$0PERI:(DE-600)2758684-4$$a10.1063/1.5091756$$gVol. 6, no. 3, p. 034301 -$$n3$$p034301$$tStructural dynamics$$v6$$x2329-7778$$y2019
000423815 8564_ $$uhttps://bib-pubdb1.desy.de/record/423815/files/1.5091756.pdf$$yOpenAccess
000423815 8564_ $$uhttps://bib-pubdb1.desy.de/record/423815/files/1.5091756.gif?subformat=icon$$xicon$$yOpenAccess
000423815 8564_ $$uhttps://bib-pubdb1.desy.de/record/423815/files/1.5091756.jpg?subformat=icon-1440$$xicon-1440$$yOpenAccess
000423815 8564_ $$uhttps://bib-pubdb1.desy.de/record/423815/files/1.5091756.jpg?subformat=icon-180$$xicon-180$$yOpenAccess
000423815 8564_ $$uhttps://bib-pubdb1.desy.de/record/423815/files/1.5091756.jpg?subformat=icon-640$$xicon-640$$yOpenAccess
000423815 8564_ $$uhttps://bib-pubdb1.desy.de/record/423815/files/1.5091756.pdf?subformat=pdfa$$xpdfa$$yOpenAccess
000423815 909CO $$ooai:bib-pubdb1.desy.de:423815$$pdnbdelivery$$pdriver$$pVDB$$popen_access$$popenaire
000423815 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1030978$$aExternal Institute$$b0$$kExtern
000423815 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1005161$$aExternal Institute$$b1$$kExtern
000423815 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1023691$$aExternal Institute$$b2$$kExtern
000423815 9101_ $$0I:(DE-H253)_CFEL-20120731$$6P:(DE-H253)PIP1030287$$aCentre for Free-Electron Laser Science$$b3$$kCFEL
000423815 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1030287$$aExternal Institute$$b3$$kExtern
000423815 9101_ $$0I:(DE-H253)_CFEL-20120731$$6P:(DE-H253)PIP1028048$$aCentre for Free-Electron Laser Science$$b4$$kCFEL
000423815 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1028048$$aExternal Institute$$b4$$kExtern
000423815 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1023228$$aExternal Institute$$b6$$kExtern
000423815 9101_ $$0I:(DE-588b)2008985-5$$6P:(DE-H253)PIP1031019$$aDeutsches Elektronen-Synchrotron$$b7$$kDESY
000423815 9101_ $$0I:(DE-588b)2008985-5$$6P:(DE-H253)PIP1025172$$aDeutsches Elektronen-Synchrotron$$b8$$kDESY
000423815 9101_ $$0I:(DE-H253)_CFEL-20120731$$6P:(DE-H253)PIP1025172$$aCentre for Free-Electron Laser Science$$b8$$kCFEL
000423815 9101_ $$0I:(DE-588b)2008985-5$$6P:(DE-H253)PIP1006748$$aDeutsches Elektronen-Synchrotron$$b9$$kDESY
000423815 9101_ $$0I:(DE-588b)2008985-5$$6P:(DE-H253)PIP1002687$$aDeutsches Elektronen-Synchrotron$$b10$$kDESY
000423815 9101_ $$0I:(DE-588b)2008985-5$$6P:(DE-H253)PIP1004087$$aDeutsches Elektronen-Synchrotron$$b11$$kDESY
000423815 9101_ $$0I:(DE-588b)2008985-5$$6P:(DE-H253)PIP1023118$$aDeutsches Elektronen-Synchrotron$$b12$$kDESY
000423815 9101_ $$0I:(DE-588b)2008985-5$$6P:(DE-H253)PIP1031146$$aDeutsches Elektronen-Synchrotron$$b13$$kDESY
000423815 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1003945$$aExternal Institute$$b14$$kExtern
000423815 9101_ $$0I:(DE-H253)_CFEL-20120731$$6P:(DE-H253)PIP1005343$$aCentre for Free-Electron Laser Science$$b15$$kCFEL
000423815 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1005343$$aExternal Institute$$b15$$kExtern
000423815 9131_ $$0G:(DE-HGF)POF3-621$$1G:(DE-HGF)POF3-620$$2G:(DE-HGF)POF3-600$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$9G:(DE-HGF)POF3-6211$$aDE-HGF$$bForschungsbereich Materie$$lVon Materie zu Materialien und Leben$$vIn-house research on the structure, dynamics and function of matter$$x0
000423815 9141_ $$y2019
000423815 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS
000423815 915__ $$0LIC:(DE-HGF)CCBY4$$2HGFVOC$$aCreative Commons Attribution CC BY 4.0
000423815 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bSTRUCT DYNAM-US : 2017
000423815 915__ $$0StatID:(DE-HGF)0501$$2StatID$$aDBCoverage$$bDOAJ Seal
000423815 915__ $$0StatID:(DE-HGF)0500$$2StatID$$aDBCoverage$$bDOAJ
000423815 915__ $$0StatID:(DE-HGF)0111$$2StatID$$aWoS$$bScience Citation Index Expanded
000423815 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection
000423815 915__ $$0StatID:(DE-HGF)9900$$2StatID$$aIF < 5
000423815 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
000423815 915__ $$0StatID:(DE-HGF)0030$$2StatID$$aPeer Review$$bDOAJ : Peer review
000423815 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences
000423815 915__ $$0StatID:(DE-HGF)0310$$2StatID$$aDBCoverage$$bNCBI Molecular Biology Database
000423815 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline
000423815 915__ $$0StatID:(DE-HGF)0320$$2StatID$$aDBCoverage$$bPubMed Central
000423815 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List
000423815 9201_ $$0I:(DE-H253)FS-FLASH-B-20160930$$kFS-FLASH-B$$lFLASH Photonen-Strahlführungen und Optiken$$x0
000423815 9201_ $$0I:(DE-H253)FS-FLASH-D-20160930$$kFS-FLASH-D$$lFLASH Photonen-Diagnose und Steuerungen$$x1
000423815 9201_ $$0I:(DE-H253)MFL-20120731$$kMFL$$lMaschinen Koordination FLASH$$x2
000423815 9201_ $$0I:(DE-H253)U_HH-20120814$$kU HH$$lUni Hamburg$$x3
000423815 9201_ $$0I:(DE-H253)CFEL-FXP-20160909$$kCFEL-FXP$$lUNI/EXP$$x4
000423815 980__ $$ajournal
000423815 980__ $$aVDB
000423815 980__ $$aI:(DE-H253)FS-FLASH-B-20160930
000423815 980__ $$aI:(DE-H253)FS-FLASH-D-20160930
000423815 980__ $$aI:(DE-H253)MFL-20120731
000423815 980__ $$aI:(DE-H253)U_HH-20120814
000423815 980__ $$aI:(DE-H253)CFEL-FXP-20160909
000423815 980__ $$aUNRESTRICTED
000423815 9801_ $$aFullTexts