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@ARTICLE{Klemke:420173,
author = {Klemke, Nicolai and Tancogne-Dejean, N. and Rossi, Giulio
Maria and Yang, Y. and Scheiba, F. and Mainz, Roland and Di
Sciacca, G. and Rubio, A. and Kärtner, Franz and Mücke, O.
D.},
title = {{P}olarization-state-resolved high-harmonic spectroscopy of
solids},
journal = {Nature Communications},
volume = {10},
issn = {2041-1723},
address = {[London]},
publisher = {Nature Publishing Group UK},
reportid = {PUBDB-2019-01359},
pages = {1319},
year = {2019},
abstract = {Attosecond metrology sensitive to sub-optical-cycle
electronic and structural dynamics is opening up new avenues
for ultrafast spectroscopy of condensed matter. Using
intense lightwaves to precisely control the fast carrier
dynamics in crystals holds great promise for next-generation
petahertz electronics and devices. The carrier dynamics can
produce high-order harmonics of the driving field extending
up into the extreme-ultraviolet region. Here, we introduce
polarization-state-resolved high-harmonic spectroscopy of
solids, which provides deeper insights into both electronic
and structural sub-cycle dynamics. Performing high-harmonic
generation measurements from silicon and quartz, we
demonstrate that the polarization states of the harmonics
are not only determined by crystal symmetries, but can be
dynamically controlled, as a consequence of the intertwined
interband and intraband electronic dynamics. We exploit this
symmetry-dynamics duality to efficiently generate coherent
circularly polarized harmonics from elliptically polarized
pulses. Our experimental results are supported by ab-initio
simulations, providing evidence for the microscopic origin
of the phenomenon.},
cin = {FS-CFEL-2},
ddc = {500},
cid = {I:(DE-H253)FS-CFEL-2-20120731},
pnm = {6211 - Extreme States of Matter: From Cold Ions to Hot
Plasmas (POF3-621) / DFG project 281310551 - SOLSTICE -
Festkörper in starken terahertz und
infrarotenTräger-Einhüllende phasenstabilen Wellenformen
(281310551) / DFG project 390715994 - EXC 2056: CUI:
Advanced Imaging of Matter (390715994) / DFG project
194651731 - EXC 1074: Hamburger Zentrum für ultraschnelle
Beobachtung (CUI): Struktur, Dynamik und Kontrolle von
Materie auf atomarer Skala (194651731) / NoMaD - The Novel
Materials Discovery Laboratory (676580) / QSpec-NewMat -
Quantum Spectroscopy: exploring new states of matter out of
equilibrium (694097)},
pid = {G:(DE-HGF)POF3-6211 / G:(GEPRIS)281310551 /
G:(GEPRIS)390715994 / G:(GEPRIS)194651731 /
G:(EU-Grant)676580 / G:(EU-Grant)694097},
experiment = {EXP:(DE-H253)CFEL-Exp-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:30899026},
UT = {WOS:000461881700024},
doi = {10.1038/s41467-019-09328-1},
url = {https://bib-pubdb1.desy.de/record/420173},
}