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@ARTICLE{ElsayedMoussa:416542,
author = {Elsayed Moussa, Mehdi and Peresypkina, Eugenia and
Virovets, Alexandr and Venus, Dominik and Balázs, Gábor
and Scheer, Manfred},
title = {{T}uning the dimensionality of organometallic–organic
hybrid polymers assembled from
$[{C}p_{2}{M}o_{2}({CO})_{4}(η^{2}-{P}_{2})]$, bipyridyl
linkers and ${A}g^{{I}}$ ions},
journal = {CrystEngComm},
volume = {20},
number = {46},
issn = {1466-8033},
address = {London},
publisher = {RSC},
reportid = {PUBDB-2018-04954},
pages = {7417 - 7422},
year = {2018},
note = {© The Royal Society of Chemistry},
abstract = {The reactions of the P$_2$ ligand complex
[Cp$_2$Mo$_2$(CO)$_4$($η^2$-P$_2$)] (Cp =C$_5$H$_5$, 1)
with Ag[Al{OC(CF$_3$)$_3$}$_4$] (Ag[TEF]) in the presence of
therigid bipyridyl linkers 1,2-di(pyridin-4-yl)ethyne (3),
4,4′-bis(pyridin-4-ylethynyl)-1,1′-biphenyl (4) and
4,4′-bipyridine (5) possessingvarious lengths are studied.
The reaction with the longer linkers (3and 4) leads to the
formation of the 1D organometallic–organichybrid polymers
[{Cp$_2$Mo$_2$(CO)$_4$($μ_4$,$η^{1:1:2:2}$-P$_2$)}$_2${Cp$_2$Mo$_2$(CO)$_4$($μ_3$,$η^{1:2:2}$-$P_2$)}$_2$($μ,η^{1:1}$-C$_{12}$H$_8$N$_2$)Ag$_2$]$_n$[TEF]$_{2n}$
(6)
and[{Cp$_2$Mo$_2$(CO)$_4$($μ_4$,$η^{1:1:2:2}$-P$_2$)}$_2${Cp$_2$Mo$_2$(CO)$_4$($μ_3$,$η^{1:2:2}$-P$_2$)}$_2$($μ,η^{1:1}$-C$_{26}$H$_{16}$N$_2$)Ag$_2$]$_n$[TEF]$_{2n}$
(7) in high selectivity. A similar reaction withthe short
linker 5 affords a mixture of the 2D hybrid
polymers[{Cp$_2$Mo$_2$(CO)$_4$($μ_4$,$η^{1:2:2:2}$-P$_2$)}$_2$($μ,η^{1:1}$-C$_{13}$H$_{14}$N$_2$)Ag$_2$]$_n$[TEF]$_{2n}$
(8) andthe 3D hybrid network
[{Cp$_2$Mo$_2$(CO)$_4$($μ_4$,$η^{1:1:2:2}$-P$_2$)}$_2$($μ,η^{1:1}$-C$_{10}$H$_8$N$_2$)Ag]$_n$[TEF]$_{2n}$
(9). However, a selective synthesis of 8 or 9 ispossible
when the reaction is performed at 0 °C and 60
°C,respectively.},
cin = {DOOR},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {6G3 - PETRA III (POF3-622) / FS-Proposal: I-20160654
(I-20160654)},
pid = {G:(DE-HGF)POF3-6G3 / G:(DE-H253)I-20160654},
experiment = {EXP:(DE-H253)P-P11-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000451535200002},
doi = {10.1039/C8CE01792A},
url = {https://bib-pubdb1.desy.de/record/416542},
}