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@ARTICLE{Heymann:408573,
      author       = {Heymann, Leonard and Schiller, Björn and Noei, Heshmat and
                      Stierle, Andreas and Klinke, Christian},
      title        = {{A} {N}ew {S}ynthesis {A}pproach for {C}arbon {N}itrides:
                      {P}oly(triazine imide) and {I}ts {P}hotocatalytic
                      {P}roperties},
      journal      = {ACS omega},
      volume       = {3},
      number       = {4},
      issn         = {2470-1343},
      address      = {Washington, DC},
      publisher    = {ACS Publications},
      reportid     = {PUBDB-2018-02965},
      pages        = {3892 - 3900},
      year         = {2018},
      abstract     = {Poly(triazine imide) (PTI) is a materialbelonging to the
                      group of carbon nitrides and has shown tohave competitive
                      properties compared to melon or g-C3N4,especially in
                      photocatalysis. As most of the carbon nitrides, PTIis
                      usually synthesized by thermal or hydrothermal approaches.We
                      present and discuss an alternative synthesis for PTI
                      whichexhibits a pH-dependent solubility in aqueous
                      solutions. Thissynthesis is based on the formation of
                      radicals duringelectrolysis of an aqueous melamine solution,
                      coupling ofresulting melamine radicals and the final
                      formation of PTI. Weapplied different characterization
                      techniques to identify PTI asthe product of this reaction
                      and report the first liquid stateNMR experiments on a
                      triazine-based carbon nitride. We showthat PTI has a
                      relatively high specific surface area and a
                      pHdependentadsorption of charged molecules. This tunable
                      adsorption has a significant influence on the photocatalytic
                      propertiesof PTI, which we investigated in dye degradation
                      experiments.},
      cin          = {UNI/PHY / DOOR / FS-NL},
      ddc          = {540},
      cid          = {$I:(DE-H253)UNI_PHY-20170505$ /
                      I:(DE-H253)HAS-User-20120731 / I:(DE-H253)FS-NL-20120731},
      pnm          = {6213 - Materials and Processes for Energy and Transport
                      Technologies (POF3-621)},
      pid          = {G:(DE-HGF)POF3-6213},
      experiment   = {EXP:(DE-H253)Nanolab-01-20150101 /
                      EXP:(DE-H253)Nanolab-02-20150101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:29732448},
      UT           = {WOS:000430200300030},
      doi          = {10.1021/acsomega.8b00294},
      url          = {https://bib-pubdb1.desy.de/record/408573},
}