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@ARTICLE{Terraschke:398019,
author = {Terraschke, Huayna and Rothe, Merrit Johanna and
Lindenberg, Patric},
title = {{I}n situ monitoring metal-ligand exchange processes by
optical spectroscopy and {X}-ray diffraction analysis: a
review},
journal = {Reviews in analytical chemistry},
volume = {37},
number = {1},
issn = {2191-0189},
address = {Berlin},
publisher = {de Gruyter},
reportid = {PUBDB-2017-13636},
pages = {20170003},
year = {2017},
abstract = {Knowledge about the mechanisms involved in the structural
development of solid materials at the atomic level is
essential for designing rational synthesis protocols for
these compounds, which may be used to improve desired
technical properties, such as light emission, conductivity,
magnetism, porosity or particle size, and may allow the
tailored design of solid materials to generate the
aforementioned properties. Recent technological advancements
have allowed the combination of synchrotron-based in situ
X-ray diffraction (XRD) with in situ optical spectroscopy
techniques, providing researchers with remarkable
opportunities to directly investigate structural changes
during synthesis reactions. Among the various available
methods to measure optical properties, in situ luminescence,
UV/Vis absorption, and light transmission spectroscopies are
highlighted here, with in situ luminescence being subdivided
into in situ luminescence analysis of coordination sensors
(ILACS) and time-resolved laser fluorescence spectroscopy
(TRLFS). This article consists of a review of 122 references
exploring various aspects of in situ analyses, with
particular emphasis on the use of XRD-combined techniques in
the study of metal-ligand exchange processes during the
formation, phase transitions and decomposition of solid
materials, including complexes, coordination polymers,
metal-organic frameworks, nanoparticles and polyoxo- or
chalcogenide metallates. We will then conclude with an
exploration of future trends in this exciting research
field.},
cin = {DOOR},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {6G3 - PETRA III (POF3-622)},
pid = {G:(DE-HGF)POF3-6G3},
experiment = {EXP:(DE-H253)P-P09-20150101 / EXP:(DE-H253)P-P07-20150101},
typ = {PUB:(DE-HGF)36 / PUB:(DE-HGF)16},
UT = {WOS:000427672600001},
doi = {10.1515/revac-2017-0003},
url = {https://bib-pubdb1.desy.de/record/398019},
}