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@ARTICLE{CercKoroec:390612,
author = {Cerc Korošec, Romana and Umek, Polona and Gloter,
Alexandre and Padežnik Gomilšek, Jana and Bukovec, Peter},
title = {{S}tructural properties and thermal stability of cobalt-
and chromium-doped $\mathrm{\alpha-{M}n{O}_{2}}$ nanorods},
journal = {Beilstein journal of nanotechnology},
volume = {8},
issn = {2190-4286},
address = {Frankfurt, M.},
publisher = {Beilstein-Institut zur Förderung der Chemischen
Wissenschaften},
reportid = {PUBDB-2017-09669},
pages = {1032 - 1042},
year = {2017},
abstract = {$\alpha$-MnO$_{2}$ nanorods were synthesized via the
hydrothermal decomposition of KMnO$_4$ in an acidic
environment in the presence of Co$^{2+}$ and Cr$^{3+}$ ions.
Reactions were carried out at three different temperatures:
90, 130 and 170 °C. All prepared samples exhibit a
tetragonal MnO$_2$ crystalline phase. SEM–EDS analysis
shows that cobalt cations are incorporated to a higher
degree into the MnO$_2$ framework than chromium ions, and
that the content of the dopant ions decreases with
increasing reaction temperature. The oxidation of Co$^{2+}$
to Co$^{3+}$ during the reaction was proved by an XANES
study, while EXAFS results confirm that both dopant ions
substitute Mn$^{4+}$ in the center of an octahedron. The
K/Mn ratio in the doped samples synthesized at 170 °C is
significantly lower than in the undoped samples. Analysis of
an individual cobalt-doped $\alpha$-MnO$_{2}$ nanorod with
HAADF-STEM reveals that the distribution of cobalt through
the cross-section of the nanorod is uniform. The course of
thermal decomposition of the doped nanorods is similar to
that of the undoped ones. Dopant ions do not preserve the
MnO$_2$ phase at higher temperatures nor do they destabilize
the cryptomelane structure.},
cin = {DOOR},
ddc = {620},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {899 - ohne Topic (POF3-899) / FS-Proposal: II-20080058 EC
(II-20080058-EC) / FS-Proposal: I-20110082 EC
(I-20110082-EC)},
pid = {G:(DE-HGF)POF3-899 / G:(DE-H253)II-20080058-EC /
G:(DE-H253)I-20110082-EC},
experiment = {EXP:(DE-H253)D-C-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000406241500001},
pubmed = {pmid:28546897},
doi = {10.3762/bjnano.8.104},
url = {https://bib-pubdb1.desy.de/record/390612},
}