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000331156 245__ $$aAlignment, Orientation, and Coulomb Explosion of Difluoroiodobenzene Studied with the Pixel Imaging Mass Spectrometry (PImMS) Camera
000331156 260__ $$c2017
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000331156 520__ $$aLaser-induced adiabatic alignment and mixed-field orientation of 2,6-difluoroiodobenzene (C$_6$H$_3$F$_2$I) molecules are probed by Coulomb explosion imaging following either near-infrared strong-field ionization or extreme-ultraviolet multi-photon inner-shell ionization using free-electron laser pulses. The resulting photoelectrons and fragment ions are captured by a double-sided velocity map imaging spectrometer and projected onto two position-sensitive detectors. The ion side of the spectrometer is equipped with the Pixel Imaging Mass Spectrometry (PImMS) camera, a time-stamping pixelated detector that can record the hit positions and arrival times of up to four ions per pixel per acquisition cycle. Thus, the time-of-flight trace and ion momentum distributions for all fragments can be recorded simultaneously. We show that we can obtain a high degree of one- and three-dimensional alignment and mixed- field orientation, and compare the Coulomb explosion process induced at both wavelengths.
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000331156 7001_ $$0P:(DE-H253)PIP1006803$$aRudenko, Artem$$b32
000331156 7001_ $$0P:(DE-HGF)0$$aStapelfeldt, Henrik$$b33
000331156 7001_ $$0P:(DE-HGF)0$$aBrouard, Mark$$b34
000331156 7001_ $$0P:(DE-H253)PIP1007320$$aRolles, Daniel$$b35$$eCorresponding author
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