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@ARTICLE{Santoso:320128,
author = {Santoso, Iman and Ku, Wei and Shirakawa, Tomonori and
Neuber, Gerd and Yin, Xinmao and Enoki, M. and Fujita,
Masaki and Liang, Ruixing and Venkatesan, T. and Sawatzky,
George A. and Kotlov, Aleksei and Yunoki, Seiji and
Rübhausen, Michael and Rusydi, Andrivo},
title = {{U}nraveling {L}ocal {S}pin {P}olarization of
{Z}hang-{R}ice {S}inglet in {L}ightly {H}ole-{D}oped
{C}uprates {U}sing {H}igh-{E}nergy {O}ptical {C}onductivity},
journal = {Physical review / B},
volume = {95},
number = {16},
issn = {2469-9950},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {PUBDB-2017-01533},
pages = {165108},
year = {2017},
abstract = {Unrevealing local magnetic and electronic correlations in
the vicinity of charge carriers is crucial in order
tounderstand rich physical properties in correlated electron
systems. Here, using high-energy optical conductivity(up to
35 eV) as a function of temperature and polarization, we
observe a surprisingly strong spin polarizationof the local
spin singlet with enhanced ferromagnetic correlations
between Cu spins near the doped holesin lightly hole-doped
$La_{1.95}Sr_{0.05}Cu_{0.95}Zn_{0.05}O_4$. The changes of
the local spin polarization manifest stronglyin the
temperature-dependent optical conductivity at ∼7.2 eV,
with an anomaly at the magnetic stripe phase(∼ 25 K),
accompanied by anomalous spectral-weight transfer in a broad
energy range. Supported by theoreticalcalculations, we also
assign high-energy optical transitions and their
corresponding temperature dependence,particularly at ∼2.5,
∼8.7, ∼9.7, ∼11.3, and ∼21.8 eV. Our result shows
the importance of a strong mixture ofspin singlet and
triplet states in hole-doped cuprates and demonstrates a new
strategy to probe local magneticcorrelations using
high-energy optical conductivity in correlated electron
systems.},
cin = {DOOR / FS-PEX / CFEL-AO},
ddc = {530},
cid = {I:(DE-H253)HAS-User-20120731 / I:(DE-H253)FS-PEX-20130206 /
I:(DE-H253)CFEL-AO-20160914},
pnm = {6213 - Materials and Processes for Energy and Transport
Technologies (POF3-621)},
pid = {G:(DE-HGF)POF3-6213},
experiment = {EXP:(DE-H253)D-I-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000402740100001},
doi = {10.1103/PhysRevB.95.165108},
url = {https://bib-pubdb1.desy.de/record/320128},
}