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000318250 0247_ $$2doi$$a10.1103/PhysRevLett.118.087403
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000318250 0247_ $$2ISSN$$a1079-7114
000318250 0247_ $$2ISSN$$a1092-0145
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000318250 1001_ $$0P:(DE-H253)PIP1028483$$aTancogne-Dejean, Nicolas$$b0$$eCorresponding author
000318250 245__ $$aImpact of the Electronic Band Structure in High-Harmonic Generation Spectra of Solids
000318250 260__ $$aCollege Park, Md.$$bAPS$$c2017
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000318250 520__ $$aAn accurate analytic model describing the microscopic mechanism of high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results reveal that (i) the emitted HHG spectra are highly anisotropic and laser-polarization dependent even for cubic crystals; (ii) the harmonic emission is enhanced by the inhomogeneity of the electron-nuclei potential; the yield is increased for heavier atoms; and (iii) the cutoff photon energy is driver-wavelength independent. Moreover, we show that it is possible to predict the laser polarization for optimal HHG in bulk crystals solely from the knowledge of their electronic band structure. Our results pave the way to better control and optimize HHG in solids by engineering their band structure.
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000318250 7001_ $$0P:(DE-H253)PIP1014908$$aMuecke, Oliver D.$$b1$$udesy
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000318250 7001_ $$0P:(DE-H253)PIP1023770$$aRubio, Angel$$b3
000318250 773__ $$0PERI:(DE-600)1472655-5$$a10.1103/PhysRevLett.118.087403$$gVol. 118, no. 8, p. 087403$$n8$$p087403$$tPhysical review letters$$v118$$x1079-7114$$y2017
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