TY - JOUR AU - Horke, Daniel AU - Chang, Yuan-Pin AU - Dlugolecki, Karol AU - Küpper, Jochen TI - Separating Para and Ortho Water JO - Angewandte Chemie / International edition VL - 53 IS - 44 SN - 1433-7851 CY - Weinheim PB - Wiley-VCH M1 - PUBDB-2017-00963 M1 - arXiv:1407.2056 SP - 11965 - 11968 PY - 2014 N1 - (c) WILEY-VCH Verlag GmbH & Co. KGaA. ; Post referee fulltext in progress; Embargo 12 months from publication AB - Water exists as two nuclear-spin isomers, para and ortho, determined by the overall spin of its two hydrogen nuclei. For isolated water molecules, the conversion between these isomers is forbidden and they act as different molecular species. Yet, these species are not readily separated, and no pure para sample has been produced. Accordingly, little is known about their specific physical and chemical properties, conversion mechanisms, or interactions. The production of isolated samples of both spin isomers is demonstrated in pure beams of para and ortho water in their respective absolute ground state. These single-quantum-state samples are ideal targets for unraveling spin-conversion mechanisms, for precision spectroscopy and fundamental symmetry-breaking studies, and for spin-enhanced applications, for example laboratory astrophysics and astrochemistry or hypersensitized NMR experiments. LB - PUB:(DE-HGF)29 ; PUB:(DE-HGF)16 UR - <Go to ISI:>//WOS:000344050700047 C6 - pmid:25196938 DO - DOI:10.1002/anie.201405986 UR - https://bib-pubdb1.desy.de/record/317924 ER -