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@ARTICLE{Gati:317888,
author = {Gati, Cornelius and Oberthuer, Dominik and Yefanov,
Oleksandr and Bunker and Stellato, Francesco and chiu,
Elaine and Yeh, Shin-Mei and Aquila, Andrew and Basu, Shibom
and Bean, Richard and Beyerlein, Kenneth and Botha, Sabine
and Boutet, Sebastien and DePonte, Daniel and Doak, R. Bruce
and Fromme, Raimund and Galli, Lorenzo and grotjohan, Ingo
and James, Daniel and Kupitz, Christopher and Lomb, Lukas
and Messerschmidt, Marc and Nass, Karol and Rendek, Kimberly
and Shoeman, Robert and Wang, Dingjie and Weierstall, Uwe
and White, Thomas and Williams, Garth and Zatsepin, Nadia
and Fromme, Petra and Goldie, Kenneth and Jehle, Johannes
and Metcalf, Peter and Barty, Anton and Chapman, Henry N.},
title = {{A}tomic {S}tructure of {G}ranulin {D}etermined from
{N}ative {N}anocrystalline {G}ranulovirus {U}sing an {X}-ray
{F}ree-{E}lectron {L}aser},
journal = {Proceedings of the National Academy of Sciences of the
United States of America},
volume = {114},
number = {9},
issn = {0027-8424},
address = {Washington, DC},
publisher = {National Acad. of Sciences},
reportid = {PUBDB-2017-00953},
pages = {2247 – 2252},
year = {2017},
note = {© National Academy of Sciences},
abstract = {To understand how molecules function in biological systems,
new methods are required to obtain atomic resolution
structures from biological material under physiological
conditions. Intense femtosecond-duration pulses from X-ray
free-electron lasers (XFELs) can outrun most damage
processes, vastly increasing the tolerable dose before the
specimen is destroyed. This in turn allows structure
determination from crystals much smaller and more radiation
sensitive than previously considered possible, allowing data
collection from room temperature structures and avoiding
structural changes due to cooling. Regardless,
high-resolution structures obtained from XFEL data mostly
use crystals far larger than 1 μm$^3$ in volume, whereas
the X-ray beam is often attenuated to protect the detector
from damage caused by intense Bragg spots. Here, we describe
the 2 Å resolution structure of native nanocrystalline
granulovirus occlusion bodies (OBs) that are less than 0.016
μm$^3$ in volume using the full power of the Linac Coherent
Light Source (LCLS) and a dose up to 1.3 GGy per crystal.
The crystalline shell of granulovirus OBs consists, on
average, of about 9,000 unit cells, representing the
smallest protein crystals to yield a high-resolution
structure by X-ray crystallography to date. The XFEL
structure shows little to no evidence of radiation damage
and is more complete than a model determined using
synchrotron data from recombinantly produced, much larger,
cryocooled granulovirus granulin microcrystals. Our
measurements suggest that it should be possible, under ideal
experimental conditions, to obtain data from protein
crystals with only 100 unit cells in volume using currently
available XFELs and suggest that single-molecule imaging of
individual biomolecules could almost be within reach.},
cin = {CFEL-I / Eur.XFEL / UNI/CUI / CFEL-QCM / ASU},
ddc = {000},
cid = {I:(DE-H253)CFEL-I-20161114 / $I:(DE-H253)Eur_XFEL-20120731$
/ $I:(DE-H253)UNI_CUI-20121230$ /
I:(DE-H253)CFEL-QCM-20160914 / I:(DE-H253)ASU-20151130},
pnm = {6215 - Soft Matter, Health and Life Sciences (POF3-621) /
Leibniz Preis - Leibiz Programm 2015: Prof. Dr. Henry N.
Chapman (DFG-Leibniz-2015-Chapman) / VH-GS-500 - PIER
Helmholtz Graduate School $(2015_IFV-VH-GS-500)$},
pid = {G:(DE-HGF)POF3-6215 / G:(DE-H253)DFG-Leibniz-2015-Chapman /
$G:(DE-HGF)2015_IFV-VH-GS-500$},
experiment = {EXP:(DE-H253)CFEL-Exp-20150101 /
EXP:(DE-MLZ)External-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000395101200053},
pubmed = {pmid:28202732},
doi = {10.1073/pnas.1609243114},
url = {https://bib-pubdb1.desy.de/record/317888},
}