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@ARTICLE{Schlathoelter:315234,
author = {Schlathoelter, Thomas and Reitsma, Geert and Egorov,
Dmitrii and Gonzalez-Magaña, Olmo and Bari, Sadia and
Boschman, Leon and Bodewits, Erwin and Schnorr, Kirsten and
Schmid, Georg and Schröter, Claus Dieter and Moshammer,
Robert and Hoekstra, Ronnie},
title = {{M}ultiple {I}onization of {F}ree {U}biquitin {M}olecular
{I}ons in {E}xtreme {U}ltraviolet {F}ree-{E}lectron {L}aser
{P}ulses},
journal = {Angewandte Chemie / International edition},
volume = {128},
number = {36},
issn = {0044-8249},
address = {Weinheim},
publisher = {Wiley-VCH9102},
reportid = {PUBDB-2016-05703},
pages = {10899 - 10903},
year = {2016},
note = {(c) WILEY-VCH Verlag GmbH $\&$ Co. KGaA},
abstract = {The fragmentation of free tenfold protonated ubiquitin in
intense 70 femtosecond pulses of 90 eV photons from the
FLASH facility was investigated. Mass spectrometric
investigation of the fragment cations produced after removal
of many electrons revealed fragmentation predominantly into
immonium ions and related ions, with yields increasing
linearly with intensity. Ionization clearly triggers a
localized molecular response that occurs before the
excitation energy equilibrates. Consistent with this
interpretation, the effect is almost unaffected by the
charge state, as fragmentation of sixfold deprotonated
ubiquitin leads to a very similar fragmentation pattern.
Ubiquitin responds to EUV multiphoton ionization as an
ensemble of small peptides.},
cin = {DOOR / FS-FLASH-O / FS-SCS},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731 /
I:(DE-H253)FS-FLASH-O-20160930 / I:(DE-H253)FS-SCS-20131031},
pnm = {6211 - Extreme States of Matter: From Cold Ions to Hot
Plasmas (POF3-621) / 6G2 - FLASH (POF3-622) / CALIPSO -
Coordinated Access to Lightsources to Promote Standards and
Optimization (312284)},
pid = {G:(DE-HGF)POF3-6211 / G:(DE-HGF)POF3-6G2 /
G:(EU-Grant)312284},
experiment = {EXP:(DE-H253)F-BL3-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:27453360},
UT = {WOS:000383473600038},
doi = {10.1002/ange.201605335},
url = {https://bib-pubdb1.desy.de/record/315234},
}