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000307321 1001_ $$0P:(DE-H253)PIP1013512$$aMitrano, M.$$b0$$eCorresponding author
000307321 245__ $$aPressure-Dependent Relaxation in the Photoexcited Mott Insulator $\mathrm{ET–F_2TCNQ}$: Influence of Hopping and Correlations on Quasiparticle Recombination Rates
000307321 260__ $$aCollege Park, Md.$$bAPS$$c2014
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000307321 520__ $$aWe measure the ultrafast recombination of photoexcited quasiparticles (holon-doublon pairs) in the one dimensional Mott insulator ET–F$_2$TCNQ as a function of external pressure, which is used to tune the electronic structure. At each pressure value, we first fit the static optical properties and extract the electronic bandwidth t and the intersite correlation energy V. We then measure the recombination times as a function of pressure, and we correlate them with the corresponding microscopic parameters. We find that the recombination times scale differently than for metals and semiconductors. A fit to our data based on the time-dependent extended Hubbard Hamiltonian suggests that the competition between local recombination and delocalization of the Mott-Hubbard exciton dictates the efficiency of the recombination.
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000307321 7001_ $$0P:(DE-H253)PIP1012176$$aCotugno, G.$$b1
000307321 7001_ $$0P:(DE-HGF)0$$aClark, S. R.$$b2
000307321 7001_ $$0P:(DE-H253)PIP1012564$$aSingla, R.$$b3
000307321 7001_ $$0P:(DE-HGF)0$$aKaiser, S.$$b4
000307321 7001_ $$0P:(DE-HGF)0$$aStähler, J.$$b5
000307321 7001_ $$0P:(DE-HGF)0$$aBeyer, R.$$b6
000307321 7001_ $$0P:(DE-H253)PIP1010755$$aDressel, M.$$b7
000307321 7001_ $$0P:(DE-HGF)0$$aBaldassarre, L.$$b8
000307321 7001_ $$0P:(DE-H253)PIP1011602$$aNicoletti, D.$$b9
000307321 7001_ $$0P:(DE-HGF)0$$aPerucchi, A.$$b10
000307321 7001_ $$0P:(DE-H253)PIP1013839$$aHasegawa, T.$$b11
000307321 7001_ $$0P:(DE-HGF)0$$aOkamoto, H.$$b12
000307321 7001_ $$0P:(DE-HGF)0$$aJaksch, D.$$b13
000307321 7001_ $$0P:(DE-H253)PIP1006448$$aCavalleri, A.$$b14
000307321 773__ $$0PERI:(DE-600)1472655-5$$a10.1103/PhysRevLett.112.117801$$gVol. 112, no. 11, p. 117801$$n11$$p117801$$tPhysical review letters$$v112$$x1079-7114$$y2014
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