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| Home > Publications database > Nonlinear Lattice Dynamics as a Basis for Enhanced Superconductivity in $YBa_2Cu_3O_{6.5}$ > print |
| 001 | 307289 | ||
| 005 | 20211110134836.0 | ||
| 024 | 7 | _ | |a 10.1038/nature13875 |2 doi |
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| 100 | 1 | _ | |a Mankowsky, R. |0 P:(DE-H253)PIP1013738 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Nonlinear Lattice Dynamics as a Basis for Enhanced Superconductivity in $YBa_2Cu_3O_{6.5}$ |
| 260 | _ | _ | |a London |c 2014 |b Macmillan28177 |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Terahertz-frequency optical pulses can resonantly drive selected vibrationalmodes in solids and deformtheir crystal structures. Incomplex oxides, this method has been used to melt electronic order, drive insulator-to-metal transitions and induce superconductivity. Strikingly, coherent interlayer transport strongly reminiscent of superconductivity can be transiently induced up to room temperature (300 kelvin) in YBa$_2$Cu$_3$O$_{6+x}$. Here we report the crystal structure of this exotic non-equilibrium state, determined by femtosecond X-ray diffraction and ab initio density functional theory calculations.We find thatnonlinear lattice excitationinnormal-state YBa$_2$Cu$_3$O$_{6+x}$ at above the transitiontemperature of 52 kelvin causes a simultaneous increase anddecrease in the Cu–O$_2$ intra-bilayer and, respectively, interbilayer distances, accompanied by anisotropic changes in the in-plane O–Cu–O bond buckling. Density functional theory calculations indicate that these motions cause drastic changes in the electronic structure. Among these, the enhancement in the d$_{x^2-y^2}$ character of the in-plane electronic structure is likely to favour superconductivity. |
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| 773 | _ | _ | |a 10.1038/nature13875 |g Vol. 516, no. 7529, p. 71 - 73 |0 PERI:(DE-600)1413423-8 |n 7529 |p 71 - 73 |t Nature |v 516 |y 2014 |x 1476-4687 |
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