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000301795 1001_ $$0P:(DE-H253)PIP1012564$$aSingla, R.$$b0$$eCorresponding author
000301795 245__ $$aTHz-Frequency Modulation of the Hubbard U in an Organic Mott Insulator
000301795 260__ $$aCollege Park, Md.$$bAPS$$c2015
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000301795 520__ $$aWe use midinfrared pulses with stable carrier-envelope phase offset to drive molecular vibrations in the charge transfer salt ET−F$_2$TCNQ, a prototypical one-dimensional Mott insulator. We find that the Mott gap, which is probed resonantly with 10 fs laser pulses, oscillates with the pump field. This observation reveals that molecular excitations can coherently perturb the electronic on-site interactions (Hubbard U) by changing the local orbital wave function. The gap oscillates at twice the frequency of the vibrational mode, indicating that the molecular distortions couple quadratically to the local charge density.
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000301795 7001_ $$0P:(DE-H253)PIP1012176$$aCotugno, G.$$b1
000301795 7001_ $$aKaiser, S.$$b2
000301795 7001_ $$0P:(DE-H253)PIP1007487$$aFörst, M.$$b3
000301795 7001_ $$0P:(DE-H253)PIP1013512$$aMitrano, M.$$b4
000301795 7001_ $$aLiu, H. Y.$$b5
000301795 7001_ $$0P:(DE-H253)PIP1016132$$aCartella, A.$$b6
000301795 7001_ $$0P:(DE-H253)PIP1009108$$aManzoni, C.$$b7
000301795 7001_ $$0P:(DE-HGF)0$$aOkamoto, H.$$b8
000301795 7001_ $$0P:(DE-H253)PIP1013839$$aHasegawa, T.$$b9
000301795 7001_ $$0P:(DE-HGF)0$$aClark, S. R.$$b10
000301795 7001_ $$0P:(DE-HGF)0$$aJaksch, D.$$b11
000301795 7001_ $$0P:(DE-H253)PIP1006448$$aCavalleri, A.$$b12
000301795 773__ $$0PERI:(DE-600)1472655-5$$a10.1103/PhysRevLett.115.187401$$gVol. 115, no. 18, p. 187401$$n18$$p187401$$tPhysical review letters$$v115$$x1079-7114$$y2015
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