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@ARTICLE{Suchomski:301703,
author = {Suchomski, Christian and Reitz, Christian and Pajic, Damir
and Jaglicic, Zvonko and Djerdj, Igor and Brezesinski,
Torsten},
title = {{L}arge-{P}ore {M}esoporous ${H}o_{3}{F}e_{5}{O}_{12}$
{T}hin {F}ilms with a {S}trong {R}oom-{T}emperature
{P}erpendicular {M}agnetic {A}nisotropy by {S}ol–{G}el
{P}rocessing},
journal = {Chemistry of materials},
volume = {26},
number = {7},
issn = {1520-5002},
address = {Washington, DC},
publisher = {American Chemical Society},
reportid = {PUBDB-2016-02805},
pages = {2337 - 2343},
year = {2014},
note = {(c) American Chemical Society},
abstract = {We report the evaporation-induced self-assembly synthesis
of large-pore mesoporous thin films of ferrimagnetic holmium
iron garnet($Ho_3Fe_5O_{12}$) from nitrate salt precursors
and a polyisobutylene-blockpoly(ethylene oxide) polymer
structure-directing agent. The phase composition, atomic
bonding configuration, and pore structure of the top surface
and the interior of the films were investigated by
microscopy, scattering, and spectroscopy techniques,
including synchrotron-based grazing incidence small-angle
X-ray scattering, X-ray photoelectron spectroscopy, X-ray
diffraction (including Rietveld refinement), and others. The
data provide evidence that the sol−gelderived material is
single-phase garnet with 27 nm diameter crystallites and few
defects after being heated to 850 °C in air, and the
continuous network of pores averaging 23 nm in diameter is
preserved to a large extent, despite a solid−solid
conversion from metastable h-HoFeO$_3$ to $Ho_3Fe_5O_{12}$
during the crystallization process. Furthermore, dc
magnetometry measurements show the thin films are
magnetically stable with a room-temperature coercivity of
∼170 Oe and exhibit an out-of-plane easy axis with a
significant perpendicular magnetic anisotropy. A strong
preference for out-of-plane magnetic alignment in
solution-processed mesostructured films is unique, making
them attractive for application in spintronics and
nanomagnetics.},
cin = {DOOR},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {899 - ohne Topic (POF3-899)},
pid = {G:(DE-HGF)POF3-899},
experiment = {EXP:(DE-H253)D-BW4-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000334572300018},
doi = {10.1021/cm5003324},
url = {https://bib-pubdb1.desy.de/record/301703},
}