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@ARTICLE{Parker:299815,
author = {Parker, Stewart F. and Adroja, Devashibhai and
Jiménez-Ruiz, Mónica and Tischer, Markus and Möbus,
Konrad and Wieland, Stefan D. and Albers, Peter},
title = {{C}haracterisation of the surface of freshly prepared
precious metal catalysts},
journal = {Physical chemistry, chemical physics},
volume = {18},
issn = {1463-9076},
address = {Cambridge},
publisher = {RSC Publ.},
reportid = {PUBDB-2016-02027},
pages = {17196-17201},
year = {2016},
abstract = {A combination of electron microscopy, X-ray and neutron
spectroscopies and computational methods has provided new
insights into the species present on the surface of freshly
prepared precious metal catalysts. The results show that in
all cases, at least half of the surface is metallic or
nearly so, with the remainder covered by oxygen, largely as
hydroxide. Water is also present and is strongly held; weeks
of pumping under high vacuum is insufficient to remove it.
The hydroxyls are reactive as shown by their reaction with
or displacement by CO and can be removed by hydrogenation.
This clearly has implications for how precious metal
catalysts are activated after preparation.},
cin = {FS-US},
ddc = {540},
cid = {I:(DE-H253)FS-US-20120731},
pnm = {6214 - Nanoscience and Materials for Information Technology
(POF3-621)},
pid = {G:(DE-HGF)POF3-6214},
experiment = {EXP:(DE-H253)D-E4-20150101 / EXP:(DE-H253)D-X1-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000379482100007},
pubmed = {pmid:26986759},
doi = {10.1039/C6CP01027J},
url = {https://bib-pubdb1.desy.de/record/299815},
}