000295216 001__ 295216
000295216 005__ 20211110133447.0
000295216 0247_ $$2datacite_doi$$a10.3204/DESY-THESIS-2016-002
000295216 037__ $$aPUBDB-2016-01132
000295216 041__ $$aEnglish
000295216 0881_ $$aDESY-THESIS-2016-002
000295216 088__ $$2DESY$$aDESY-THESIS-2016-002
000295216 1001_ $$0P:(DE-H253)PIP1014316$$aRompotis, Dimitrios$$b0$$eCorresponding author$$gmale
000295216 245__ $$aA single-shot nonlinear autocorrelation approach for time-resolved physics in the vacuum ultraviolet spectral range$$f2011-04-16 - 2015-01-01
000295216 260__ $$aHamburg$$bVerlag Deutsches Elektronen-Synchrotron$$c2016
000295216 300__ $$a179
000295216 3367_ $$2DataCite$$aOutput Types/Dissertation
000295216 3367_ $$0PUB:(DE-HGF)3$$2PUB:(DE-HGF)$$aBook$$mbook
000295216 3367_ $$2ORCID$$aDISSERTATION
000295216 3367_ $$2BibTeX$$aPHDTHESIS
000295216 3367_ $$02$$2EndNote$$aThesis
000295216 3367_ $$0PUB:(DE-HGF)29$$2PUB:(DE-HGF)$$aReport$$mreport
000295216 3367_ $$0PUB:(DE-HGF)11$$2PUB:(DE-HGF)$$aDissertation / PhD Thesis$$bphd$$mphd$$s1526995842_16609
000295216 3367_ $$2DRIVER$$adoctoralThesis
000295216 4900_ $$0PERI:(DE-600)1437131-5$$aDESY-THESIS$$x1435-8085
000295216 502__ $$aDissertation, Universität Hamburg, 2015$$bDissertation$$cUniversität Hamburg$$d2015
000295216 520__ $$aIn this work, a single-shot temporal metrology scheme operating in the vacuum-extreme ultraviolet spectral range has been designed and experimentally implemented. Utilizing an anti-collinear geometry, a second-order intensity autocorrelation measurement of a vacuum ultraviolet pulse can be performed by encoding temporal delay information on the beam propagation coordinate. An ion-imaging time-of-flight spectrometer, offering micrometer resolution has been set-up for this purpose. This instrument enables the detection of a magnified image of the spatial distribution of ions exclusively generated by direct two photon absorption in the combined counter-propagating pulse focus and thus obtain the second-order intensity autocorrelation measurement on a single-shot basis.Additionally, an intense VUV light source based on high-harmonic generation has been experimentally realized. It delivers intense sub-20 fs Ti:Sa fifth-harmonic pulses utilizing a loose-focusing geometry in a long Ar gas cell. The VUV pulses centered at 161.8 nm reach pulse energies of 1.1 μJ per pulse, while the corresponding pulse duration is measured with a second-order, fringe-resolved autocorrelation scheme to be 18 ± 1 fs on average. Non-resonant, two-photon ionization of Kr and Xe and three-photon ionization of Ne verify the fifth-harmonic pulse intensity and indicate the feasibility of multi-photon VUV pump/VUV probe studies of ultrafast atomic and molecular dynamics. Finally, the extended functionality of the counter-propagating pulse metrology approach is demonstrated by a single-shot VUV pump/VUV probe experiment aiming at the investigation of ultrafast dissociation dynamics of molecular oxygen excited in the Schumann-Runge continuum at 162 nm.
000295216 536__ $$0G:(DE-HGF)POF3-6211$$a6211 - Extreme States of Matter: From Cold Ions to Hot Plasmas (POF3-621)$$cPOF3-621$$fPOF III$$x0
000295216 650_7 $$xDiss.
000295216 693__ $$0EXP:(DE-MLZ)NOSPEC-20140101$$5EXP:(DE-MLZ)NOSPEC-20140101$$eNo specific instrument$$x0
000295216 7001_ $$0P:(DE-H253)PIP1003945$$aDrescher, Markus$$b1$$eThesis advisor
000295216 8564_ $$uhttps://bib-pubdb1.desy.de/record/295216/files/Rompotis_D_PhD%20Thesis.pdf$$yOpenAccess
000295216 8564_ $$uhttps://bib-pubdb1.desy.de/record/295216/files/Rompotis_D_PhD_pdfa.pdf$$yOpenAccess
000295216 8564_ $$uhttps://bib-pubdb1.desy.de/record/295216/files/desy-thesis-16-002.title.pdf$$yOpenAccess
000295216 8564_ $$uhttps://bib-pubdb1.desy.de/record/295216/files/Rompotis_D_PhD%20Thesis.gif?subformat=icon$$xicon$$yOpenAccess
000295216 8564_ $$uhttps://bib-pubdb1.desy.de/record/295216/files/Rompotis_D_PhD%20Thesis.jpg?subformat=icon-1440$$xicon-1440$$yOpenAccess
000295216 8564_ $$uhttps://bib-pubdb1.desy.de/record/295216/files/Rompotis_D_PhD%20Thesis.jpg?subformat=icon-180$$xicon-180$$yOpenAccess
000295216 8564_ $$uhttps://bib-pubdb1.desy.de/record/295216/files/Rompotis_D_PhD%20Thesis.jpg?subformat=icon-640$$xicon-640$$yOpenAccess
000295216 8564_ $$uhttps://bib-pubdb1.desy.de/record/295216/files/Rompotis_D_PhD%20Thesis.jpg?subformat=icon-700$$xicon-700$$yOpenAccess
000295216 8564_ $$uhttps://bib-pubdb1.desy.de/record/295216/files/Rompotis_D_PhD_pdfa.gif?subformat=icon$$xicon$$yOpenAccess
000295216 8564_ $$uhttps://bib-pubdb1.desy.de/record/295216/files/Rompotis_D_PhD_pdfa.jpg?subformat=icon-180$$xicon-180$$yOpenAccess
000295216 8564_ $$uhttps://bib-pubdb1.desy.de/record/295216/files/Rompotis_D_PhD_pdfa.jpg?subformat=icon-700$$xicon-700$$yOpenAccess
000295216 8564_ $$uhttps://bib-pubdb1.desy.de/record/295216/files/desy-thesis-16-002.title.gif?subformat=icon$$xicon$$yOpenAccess
000295216 8564_ $$uhttps://bib-pubdb1.desy.de/record/295216/files/desy-thesis-16-002.title.jpg?subformat=icon-180$$xicon-180$$yOpenAccess
000295216 8564_ $$uhttps://bib-pubdb1.desy.de/record/295216/files/desy-thesis-16-002.title.jpg?subformat=icon-700$$xicon-700$$yOpenAccess
000295216 8564_ $$uhttps://bib-pubdb1.desy.de/record/295216/files/desy-thesis-16-002.title.pdf?subformat=pdfa$$xpdfa$$yOpenAccess
000295216 909CO $$ooai:bib-pubdb1.desy.de:295216$$pdnbdelivery$$pdriver$$pVDB$$popen_access$$popenaire
000295216 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1014316$$aExternes Institut$$b0$$kExtern
000295216 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1003945$$aExternes Institut$$b1$$k>Extern
000295216 9131_ $$0G:(DE-HGF)POF3-621$$1G:(DE-HGF)POF3-620$$2G:(DE-HGF)POF3-600$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$9G:(DE-HGF)POF3-6211$$aDE-HGF$$bForschungsbereich Materie$$lVon Materie zu Materialien und Leben$$vIn-house research on the structure, dynamics and function of matter$$x0
000295216 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
000295216 920__ $$lyes
000295216 9201_ $$0I:(DE-H253)UNI_EXP-20120731$$kUNI/EXP$$lUni Hamburg / Experimentalphysik$$x0
000295216 9201_ $$0I:(DE-H253)FS-FL-20120731$$kFS-FL$$lExperimentebetreuung FLASH$$x1
000295216 980__ $$aphd
000295216 980__ $$aVDB
000295216 980__ $$abook
000295216 980__ $$areport
000295216 980__ $$aI:(DE-H253)UNI_EXP-20120731
000295216 980__ $$aI:(DE-H253)FS-FL-20120731
000295216 980__ $$aUNRESTRICTED
000295216 9801_ $$aFullTexts