TY - JOUR
AU - Helml, W.
AU - Maier, A. R.
AU - Schweinberger, W.
AU - Grguraš, I.
AU - Radcliffe, P.
AU - Doumy, G.
AU - Roedig, C.
AU - Gagnon, J.
AU - Messerschmidt, M.
AU - Schorb, S.
AU - Bostedt, C.
AU - Grüner, F.
AU - DiMauro, L. F.
AU - Cubaynes, D.
AU - Bozek, J. D.
AU - Tschentscher, Thomas
AU - Costello, J. T.
AU - Meyer, Michael
AU - Coffee, R.
AU - Duesterer, Stefan
AU - Cavalieri, A. L.
AU - Kienberger, R.
TI - Measuring the temporal structure of few-femtosecond free-electron laser X-ray pulses directly in the time domain
JO - Nature photonics
VL - 8
IS - 12
SN - 1749-4893
CY - London [u.a.]
PB - Nature Publ. Group
M1 - PUBDB-2015-01020
SP - 950 - 957
PY - 2014
N1 - (c) Macmillan Publishers Limited. Post referee full text in progress. Embargo full text 6 months from 24 November 2014.
AB - Short-wavelength free-electron lasers are now well established as essential and unrivalled sources of ultrabright coherent X-ray radiation. One of the key characteristics of these intense X-ray pulses is their expected few-femtosecond duration. No measurement has succeeded so far in directly determining the temporal structure or even the duration of these ultrashort pulses in the few-femtosecond range. Here, by deploying the so-called streaking spectroscopy technique at the Linac Coherent Light Source, we demonstrate a non-invasive scheme for temporal characterization of X-ray pulses with sub-femtosecond resolution. This method is independent of photon energy, decoupled from machine parameters, and provides an upper bound on the X-ray pulse duration. We measured the duration of the shortest X-ray pulses currently available to be on average no longer than 4.4 fs. Analysing the pulse substructure indicates a small percentage of the free-electron laser pulses consisting of individual high-intensity spikes to be on the order of hundreds of attoseconds.
LB - PUB:(DE-HGF)16
UR - <Go to ISI:>//WOS:000345818600015
DO - DOI:10.1038/nphoton.2014.278
UR - https://bib-pubdb1.desy.de/record/206556
ER -