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000206543 1001_ $$0P:(DE-HGF)0$$aMetwalli, E.$$b0
000206543 245__ $$aPolymer-Coated PtCo Nanoparticles Deposited on Diblock Copolymer Templates: Chemical Selectivity versus Topographical Effects
000206543 260__ $$aWeinheim$$bWiley-VCH Verl.$$c2014
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000206543 520__ $$aMetal–polymer hybrid films are prepared by deposition of polymer-coated PtCo nanoparticles onto block copolymer templates. For templating, a thin film of the lamella-forming diblock copolymer poly(styrene-b-methyl methacrylate) P(S-b-MMA) is chemically etched and a topographical surface relief with 3 nm height difference is created. Two types of polymer-grafted PtCo nanoparticles are compared to explore the impact of chemical selectivity versus the topographical effect of the nanotemplate. A preferable wetting of the polystyrene (PS) domains with poly(styrenesulfonate) (PSS)-coated PtCo nanoparticles (instead of residing in the space between the domains) is observed. Our investigation reveals that the interaction between PSS-coated nanoparticles and PS domains dominates over the topographical effects of the polymer surface. In contrast, a non-selective deposition of poly(N-vinyl-2-pyrrolidone) (PVP)-coated PtCo nanoparticles and the formation of large metal-particle aggregates on the film is observed.
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000206543 7001_ $$0P:(DE-HGF)0$$aKrisch, I.$$b1
000206543 7001_ $$0P:(DE-HGF)0$$aMarkovits, I.$$b2
000206543 7001_ $$0P:(DE-HGF)0$$aRawolle, M.$$b3
000206543 7001_ $$0P:(DE-HGF)0$$aRuderer, M. A.$$b4
000206543 7001_ $$0P:(DE-HGF)0$$aGuo, S.$$b5
000206543 7001_ $$0P:(DE-HGF)0$$aWyrzgol, S.$$b6
000206543 7001_ $$0P:(DE-HGF)0$$aJentys, A.$$b7
000206543 7001_ $$0P:(DE-H253)PIP1007827$$aPerlich, Jan$$b8
000206543 7001_ $$0P:(DE-HGF)0$$aLercher, J. A.$$b9
000206543 7001_ $$0P:(DE-HGF)0$$aMüller-Buschbaum, P.$$b10$$eCorresponding Author
000206543 773__ $$0PERI:(DE-600)2025223-7$$a10.1002/cphc.201402047$$gVol. 15, no. 11, p. 2236 - 2239$$n11$$p2236 - 2239$$tChemPhysChem$$v15$$x1439-4235$$y2014
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