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000205893 1001_ $$0P:(DE-HGF)0$$aPospisilova, Aneta$$b0$$eCorresponding Author
000205893 245__ $$aGlycogen-graft-poly(2-alkyl-2-oxazolines) - The new Versatile Biopolymer-Based Thermoresponsive Macromolecular Toolbox
000205893 260__ $$aLondon$$bRSC Publishing$$c2014
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000205893 520__ $$ahis study is focused on thermoresponsive glycogen-graft-poly(2-alkyl-2-oxazolines), a new group of nanostructured hybrid dendrimeric stimuli-responsive polymers connecting the body's own biodegradable polysaccharidic dendrimer glycogen with the widely tuneable thermoresponsive behavior of polypeptide-analogic poly(2-alkyl-2-oxazolines), which are known to be biocompatible. Glycogen-graft-poly(2-alkyl-2-oxazolines) were prepared by a simple one-pot two-step procedure involving cationic ring-opening polymerization of 2-alkyl-2-oxazolines followed by termination of the living cationic ends with sodium glycogenate. As confirmed by light and X-ray scattering, as well as cryo-transmission electron microscopy, the grafted dendrimer structure allows easy adjustment of the cloud point temperature, the concentration dependence and nanostructure of the self-assembled phase separated polymer by crosstalk during graft composition, the graft length and the grafting density, in a very wide range.
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000205893 7001_ $$0P:(DE-H253)PIP1012775$$aFilippov, Sergey$$b1
000205893 7001_ $$0P:(DE-H253)PIP1020385$$aBogomolova, Anna$$b2
000205893 7001_ $$0P:(DE-HGF)0$$aTurner, Stuart$$b3
000205893 7001_ $$0P:(DE-HGF)0$$aSedlacek, Ondrej$$b4
000205893 7001_ $$0P:(DE-HGF)0$$aMatushkin, Nikolai$$b5
000205893 7001_ $$0P:(DE-HGF)0$$aCernochova, Zulfia$$b6
000205893 7001_ $$0P:(DE-HGF)0$$aStepanek, Petr$$b7
000205893 7001_ $$0P:(DE-HGF)0$$aHruby, Martin$$b8
000205893 773__ $$0PERI:(DE-600)2623224-8$$a10.1039/c4ra10315g$$p61580-61588$$tRSC Advances$$v4$$x2046-2069$$y2014
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