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@ARTICLE{With:205635,
      author       = {With, Sebastian and Trebbin, Martin and Bartz, Christian B.
                      A. and Neuber, Christian and Dulle, Martin and Yu, Shun and
                      Roth, Stephan and Schmidt, Hans-Werner and Foerster,
                      Stephan},
      title        = {{F}ast {D}iffusion-{L}imited {L}yotropic {P}hase
                      {T}ransitions {S}tudied in {S}itu {U}sing {C}ontinuous
                      {F}low {M}icrofluidics/{M}icrofocus-{SAXS}},
      journal      = {Langmuir},
      volume       = {30},
      number       = {42},
      issn         = {0743-7463},
      address      = {Washington, DC},
      publisher    = {ACS Publ.},
      reportid     = {PUBDB-2015-00195},
      pages        = {12494 - 12502},
      year         = {2014},
      note         = {(c) American Chemical Society. Post referee full text in
                      progress. Embargo 1 Jahr ab September 12, 2014.},
      abstract     = {Fast concentration-induced diffusion-limited lyotropic
                      phase transitions can be studied in situ with millisecond
                      time resolution using continuous flow microfluidics in
                      combination with microfocus small-angle X-ray scattering.
                      The method was applied to follow a classical selfassembly
                      sequence where amphiphiles assemble into micelles, which
                      subsequently assemble into an ordered lattice via a
                      disorder/order transition. As a model system we selected the
                      self-assembly of an amphiphilic block copolymer induced by
                      the addition of a nonsolvent. Using microchannel
                      hydrodynamic flow-focusing, large concentration gradients
                      can be generated, leading to a deep quench from the miscible
                      to the microphase-separated state. Within milliseconds the
                      block copolymers assembly via a spinodal microphase
                      separation into micelles, followed by a disorder/order
                      transition into an FCC liquid-crystalline phase with
                      late-stage domain growth and shear-induced domain
                      orientation into a mesocrystal. A comparison with a slow
                      macroscopic near-equilibrium kinetic experiment shows that
                      the fast structural transitions follow a direct pathway to
                      the equilibrium structure without the trapping of metastable
                      states.},
      cin          = {DOOR},
      ddc          = {670},
      cid          = {I:(DE-H253)HAS-User-20120731},
      pnm          = {PETRA Beamline P03 (POF2-54G14) / STREAM - Structural
                      evolution at the nano- and mesoscale (291211)},
      pid          = {G:(DE-H253)POF2-P03-20130405 / G:(EU-Grant)291211},
      experiment   = {EXP:(DE-H253)P-P03-20150101},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000347744100005},
      pubmed       = {pmid:25216394},
      doi          = {10.1021/la502971m},
      url          = {https://bib-pubdb1.desy.de/record/205635},
}