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@INPROCEEDINGS{Appel:205325,
author = {Appel, Karen and Borchert, Manuela and Morgenroth, Wolfgang
and Nakatsutsumi, Motoaki and Petitgirard, Sylvain and
Priebe, Gerd and Tschentscher, Thomas and Wilke, Max},
title = {{N}ew {P}erspectives for {L}ower {M}antle {R}eaction
{M}echanism {R}esearch using {M}odern {X}-{R}ay {S}ources},
reportid = {PUBDB-2014-04726},
year = {2014},
abstract = {Chemical composition of the Earth's mantle phases have a
major effect on their stabilities and consequently on their
reactions. Especially concerning light elements and trace
elements, compositions of phases in the lower mantle remain
basically unknown because the phases are not accessible and
cannot be studied directly. In order to betterlearn about
reactions of mantle phases, related redistribution processes
of elements and the resulting properties of the mantle,
mantle phases have been studied by in-situ methods.Within
the past years, laser-heated diamond anvil cells have been
combined with synchrotron radiation induced methods to study
chemical reactions by in-situ x-ray fluorescence analysis
and combined x-ray diffraction (XRD) (Petitgirard et al.,
2012). Synchrotron radiation provides sufficiently small
spot sizes, hard x-rays and a high sensitivity.Chemical and
structural information were obtained at temperatures of up
to 4200 K and pressures up to 130 GPa. First time-resolved
measurements have been made with the objective to follow
reaction mechanisms. For XRD, a time-resolution of msec
could be achieved by single shot pulsed laser heating
(Goncharov et al., 2011), while for insituXRF studies, the
time-resolution is currently limited to the sec regime. It
is either limited by detector speed or sensitivity or
both.An alternative method to study reactions of lower
mantle phases are laser-driven shock and ramp compression
experiments. The samples are generally pumped with an
long-pulse optical laser and then probed with an x-ray
source at a delayed period. Combined with x-ray free
electron lasers as a probe beam, these experiments offer the
uniquepossibility to study reactions at a rate of up to MHz
due to the x-ray timing structure and the increased number
of photons. The High Energy Density science instrument at
the European XFEL (HED) will provide unique possibilities
for research at extreme states of matter. The instrument is
one of the six baseline instruments at the European XFEL
andwill start user operation in the second half 2017.In this
presentation, we will show results from in-situ experiments
at conditions in the lower mantle at currently available
sources and discuss the persectives to study reaction
mechanisms at such conditions at the upcoming HED
instrument.},
month = {Sep},
date = {2014-09-21},
organization = {Jahrestagung der Deutschen
Mineralogischen Gesellschaft, Jena
(Germany), 21 Sep 2014 - 24 Sep 2014},
cin = {Eur.XFEL},
cid = {$I:(DE-H253)Eur_XFEL-20120731$},
pnm = {Experiments at XFEL (POF2-54G17) / PETRA Beamline P02.2
(POF2-54G14)},
pid = {G:(DE-H253)POF2-XFEL-Exp.-20130405 /
G:(DE-H253)POF2-P02.2-20140410},
experiment = {EXP:(DE-H253)XFEL-Exp-20150101 /
EXP:(DE-H253)P-P02.2-20150101},
typ = {PUB:(DE-HGF)6},
url = {https://bib-pubdb1.desy.de/record/205325},
}