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@ARTICLE{Valant:192939,
author = {Valant, Matjaz and Arcon, Iztok and Mikulska, Iuliia and
Lisjak, Darja},
title = {{C}ation {O}rder-{D}isorder {T}ransition in {F}e-{D}oped
$6{H}-{B}a{T}i{O}_{3}$ for {D}ilute {R}oom-{T}emperature
{F}erromagnetism},
journal = {Chemistry of materials},
volume = {25},
number = {17},
issn = {0897-4756},
address = {Washington, DC},
publisher = {American Chemical Society},
reportid = {PUBDB-2014-04423},
pages = {3544 - 3550},
year = {2013},
note = {© American Chemical Society},
abstract = {Understanding the fundamental spin coupling mechanisms
indilute magnetic oxides is not possible without exact
atomistic understanding ofthe solids. This is even more
important for few systems that show diluteferromagnetism at
room temperature and could potentially be used in
spintronicand multiferroic technologies. Here, we show the
first known example of a cationordering in hexagonal
6H-perovskites. Fe3+ ions in Fe-doped 6H-BaTiO3 areinitially
randomly distributed over two Ti4+ crystallographic sites
but can be, by aprolonged heat treatment, ordered onto one
of the sites. The cation ordering isdriven by reduction in
the electrostatic repulsion, which occurs when
Fe3+substitutes the highly charged Ti4+ ions that are
located at unusual proximity toeach other. We show that such
a continuous order−disorder transition isassociated with
induction of the room-temperature dilute ferromagnetism.},
cin = {DOOR},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {DORIS Beamline C (POF2-54G13) / FS-Proposal: I-20110082 EC
(I-20110082-EC) / CALIPSO - Coordinated Access to
Lightsources to Promote Standards and Optimization (312284)},
pid = {G:(DE-H253)POF2-C-20130405 / G:(DE-H253)I-20110082-EC /
G:(EU-Grant)312284},
experiment = {EXP:(DE-H253)D-C-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000330097900019},
doi = {10.1021/cm402353t},
url = {https://bib-pubdb1.desy.de/record/192939},
}