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| 001 | 192610 | ||
| 005 | 20250730144912.0 | ||
| 024 | 7 | _ | |2 doi |a 10.1103/PhysRevB.90.014415 |
| 024 | 7 | _ | |2 ISSN |a 0163-1829 |
| 024 | 7 | _ | |2 ISSN |a 0556-2805 |
| 024 | 7 | _ | |2 ISSN |a 1095-3795 |
| 024 | 7 | _ | |2 ISSN |a 1098-0121 |
| 024 | 7 | _ | |2 ISSN |a 1550-235X |
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| 100 | 1 | _ | |0 P:(DE-H253)PIP1020413 |a Zhang, Jian |b 0 |e Corresponding Author |
| 245 | _ | _ | |a Transformation between spin-Peierls and incommensurate fluctuating phases of Sc-doped TiOCl |
| 260 | _ | _ | |a College Park, Md. |b APS |c 2014 |
| 336 | 7 | _ | |0 0 |2 EndNote |a Journal Article |
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| 336 | 7 | _ | |2 BibTeX |a ARTICLE |
| 520 | _ | _ | |a Single crystals of ScxTi1−xOCl(x=0.005) have been grown by the vapor phase transport technique. Specific heat measurements prove the absence of phase transitions for 4–200 K. Instead, an excess entropy is observed over a range of temperatures that encompasses the incommensurate phase transition at 90 K and the spin-Peierls transition at 67 K of pure TiOCl. Temperature-dependent x-ray diffraction on ScxTi1−xOCl gives broadened diffraction maxima at incommensurate positions between Tc1=61.5(3) and ∼90 K, and at commensurate positions below 61.5 K. These results are interpreted as due to the presence of an incommensurate phase without long-range order at intermediate temperatures, and of a highly disturbed commensurate phase without long-range order at low temperatures. The commensurate phase is attributed to a fluctuating spin-Peierls state on an orthorhombic lattice. The monoclinic symmetry and local structure of the fluctuations are equal to the symmetry and structure of the ordered spin-Peierls state of TiOCl. A novel feature of ScxTi1−xOCl(x=0.005) is a transformation from one fluctuating phase (the incommensurate phase at intermediate temperatures) to another fluctuating phase (the spin-Peierls-like phase). This transformation is not a phase transition occurring at a critical temperature, but it proceeds gradually over a temperature range of ∼10 K wide. The destruction of long-range order requires much lower levels of doping in TiOCl than in other low-dimensional electronic crystals, like the canonical spin-Peierls compound CuGeO3. An explanation for the higher sensitivity to doping has not been found, but it is noticed that it may be the result of an increased two-dimensional character of the doped magnetic system. The observed fluctuating states with long correlation lengths are reminiscent of Kosterlitz–Thouless-type phases in two-dimensional systems. |
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| 700 | 1 | _ | |0 P:(DE-H253)PIP1008710 |a Wölfel, Alexander |b 1 |
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| 700 | 1 | _ | |0 P:(DE-H253)PIP1008136 |a van Smaalen, Sander |b 4 |
| 700 | 1 | _ | |0 P:(DE-HGF)0 |a Kremer, Reinhard K. |b 5 |
| 700 | 1 | _ | |0 P:(DE-HGF)0 |a Williamson, Hailey L. |b 6 |
| 773 | 1 | 8 | |a 10.1103/physrevb.90.014415 |b American Physical Society (APS) |d 2014-07-15 |n 1 |p 014415 |3 journal-article |2 Crossref |t Physical Review B |v 90 |y 2014 |x 1098-0121 |
| 773 | _ | _ | |a 10.1103/PhysRevB.90.014415 |g Vol. 90, no. 1, p. 014415 |0 PERI:(DE-600)2844160-6 |n 1 |p 014415 |t Physical review / B |v 90 |y 2014 |x 1098-0121 |
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| 999 | C | 5 | |1 G. Gruner |y 1994 |2 Crossref |t Density Waves in Solids |o G. Gruner Density Waves in Solids 1994 |
| 999 | C | 5 | |1 J. W. Bray |y 1983 |2 Crossref |t Extended Linear Chain Compounds |o J. W. Bray Extended Linear Chain Compounds 1983 |
| 999 | C | 5 | |a 10.1103/PhysRevLett.71.4059 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevLett.74.1450 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevLett.79.503 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevB.58.8202 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevB.30.4297 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevB.67.020405 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevLett.70.3651 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1088/0953-8984/5/13/014 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevB.72.020105 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevB.83.180414 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevB.78.014433 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevB.81.024411 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevLett.104.146402 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevB.83.134411 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevB.71.100405 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevB.72.012420 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1002/zaac.19582950314 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevB.77.094117 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevB.80.144416 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevB.73.214410 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1103/PhysRevB.73.172413 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |1 V. Petricek |y 2006 |2 Crossref |t The Crystallographic Computing System |o V. Petricek The Crystallographic Computing System 2006 |
| 999 | C | 5 | |a 10.1107/S0108767310042297 |9 -- missing cx lookup -- |2 Crossref |
| 999 | C | 5 | |a 10.1093/acprof:oso/9780199577224.001.0001 |1 H. Nishimori |2 Crossref |9 -- missing cx lookup -- |y 2011 |
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