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@ARTICLE{Schweinefuss:192607,
author = {Schweinefuss, Maria and Baburin, Igor A. and Schroeder,
Christian and Näther, Christian and Leoni, Stefano and
Wiebcke, Michael},
title = {{I}ndium {I}midazolate {F}rameworks with {D}ifferently
{D}istorted ${R}e{O}_{3}$-{T}ype {S}tructures: {S}yntheses,
{S}tructures, {P}hase {T}ransitions, and {C}rystallization
{S}tudies},
journal = {Crystal growth $\&$ design},
volume = {14},
number = {9},
issn = {1528-7483},
address = {Washington, DC},
publisher = {ACS Publ.},
reportid = {PUBDB-2014-04189},
pages = {4664-4673},
year = {2014},
abstract = {Three indium imidazolates have been preparedby employing
solvothermal, ionothermal, and solventlesssyntheses. The
crystal structures have been determined usinglaboratory
powder XRD methods in combination with DFTcalculations. In
phases I−III, octahedrally coordinated In(III)ions are
bridged by imidazolate (im) ligands into 3Dframeworks that
are related to distorted filled-ReO3 (ABX3perovskite)
structures with different octahedron tilting.Clathrate-type
phases I (cubic space group Im3̅) and II(trigonal R3̅) may
be formulated as [A′A″3In4(im)12] andcontain two types
of cubic cages, A′ and A″, which may hostguest molecules
and are occupied by im moieties, respectively. A reversible
structural phase transition between low-temperaturephase II
and high-temperature phase I, occurring on heating at about
90 °C, was studied by DSC and variable-temperaturepowder
XRD experiments. Depending on the synthesis, more
specifically on the nature and amount of guests trapped in
the A′cages, the phase transition was suppressible,
enabling I to be recovered at room temperature. Phase III
(trigonal R3̅) may beformulated as [AIn(im)3]. It is a
dense phase in which the cubic A cages are occupied by im
moieties. For the first time, theionothermal formation of a
coordination polymer, phase III, was monitored in situ by
time-resolved EDXRD experiments. Rateconstants and
activation energies for both nucleation and crystal growth,
as estimated by kinetic analysis of the EDXRD data,
arecompared to corresponding values reported previously for
the solvothermal crystallization of other coordination
polymers.},
cin = {DOOR},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {DORIS Beamline F3 (POF2-54G13) / FS-Proposal: I-20110615
(I-20110615)},
pid = {G:(DE-H253)POF2-F3-20130405 / G:(DE-H253)I-20110615},
experiment = {EXP:(DE-H253)D-F3-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000341226500051},
doi = {10.1021/cg5007499},
url = {https://bib-pubdb1.desy.de/record/192607},
}