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| Home > Publications database > Electron Rearrangement Dynamics in Dissociating $\mathrm{I^n_2{^+}}$ Molecules Accessed by Extreme Ultraviolet Pump-Probe Experiments > print |
| 001 | 172328 | ||
| 005 | 20250717112608.0 | ||
| 024 | 7 | _ | |a 10.1103/PhysRevLett.113.073001 |2 doi |
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| 024 | 7 | _ | |a 1079-7114 |2 ISSN |
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| 037 | _ | _ | |a PUBDB-2014-03678 |
| 041 | _ | _ | |a English |
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| 100 | 1 | _ | |a Schnorr, K. |0 P:(DE-H253)PIP1013918 |b 0 |e Corresponding Author |
| 245 | _ | _ | |a Electron Rearrangement Dynamics in Dissociating $\mathrm{I^n_2{^+}}$ Molecules Accessed by Extreme Ultraviolet Pump-Probe Experiments |
| 260 | _ | _ | |a College Park, Md. |c 2014 |b APS |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a The charge rearrangement in dissociating In+2 molecules is measured as a function of the internuclear distance R using extreme ultraviolet pulses delivered by the free-electron laser in Hamburg. Within an extreme ultraviolet pump-probe scheme, the first pulse initiates dissociation by multiply ionizing I2, and the delayed probe pulse further ionizes one of the two fragments at a given time, thus triggering charge rearrangement at a well-defined R. The electron transfer between the fragments is monitored by analyzing the delay-dependent ion kinetic energies and charge states. The experimental results are in very good agreement with predictions of the classical over-the-barrier model demonstrating its validity in a thus far unexplored quasimolecular regime relevant for free-electron laser, plasma, and chemistry applications. |
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| 773 | _ | _ | |a 10.1103/PhysRevLett.113.073001 |g Vol. 113, no. 7, p. 073001 |0 PERI:(DE-600)1472655-5 |n 7 |p 073001 |t Physical review letters |v 113 |y 2014 |x 1079-7114 |
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