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@ARTICLE{Ebbinghaus:168894,
author = {Ebbinghaus, Stefan G. and Krause, Holger and Lee, Doh-Kwon
and Janek, Jürgen},
title = {{S}ingle {C}rystals of {C}12{A}7
$\mathrm{({C}a_{12}{A}l_{14}{O}_{33})}$ {S}ubstituted with 1
mol \% {I}ron},
journal = {Crystal growth $\&$ design},
volume = {14},
number = {5},
issn = {1528-7505},
address = {Washington, DC},
publisher = {ACS Publ.},
reportid = {DESY-2014-02712},
pages = {2240 - 2245},
year = {2014},
abstract = {Single crystals of Ca12Al14O33 (C12A7, mayenite)
substituted with 1 mol $\%$ Fe were grown by the floating
zone technique in an atmosphere of $2\%$ $O2/98\%$ N2. The
iron substitution leads to an increase of the unit cell
parameter by roughly 0.002 Å. Optical spectroscopy reveals
an additional broad absorption band at 310 nm for the
iron-substituted sample reflecting the yellow color of the
crystals. XANES measurements at the Fe–K absorption edge
prove the incorporation of Fe3+ on the aluminum sites.
Measurements of the magnetic susceptibility resulted in a
value of 5.8 μB per iron ion as expected for high-spin
Fe3+. C12A7 is known to be a very good oxygen ion conductor
at high temperatures. In pure oxygen, the iron substitution
leads to a slightly reduced conductivity between
approximately 500 and 800 °C, while at higher temperatures,
the conductivity is very similar to the pristine material.
Under reducing conditions, the slope of log(σ) vs
log(p(O2)) of the iron-substituted sample was found to be
steeper than that for pure C12A7.},
cin = {DOOR},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {DORIS Beamline A1 (POF2-54G13) / FS-Proposal: I-20110471
(I-20110471)},
pid = {G:(DE-H253)POF2-A1-20130405 / G:(DE-H253)I-20110471},
experiment = {EXP:(DE-H253)D-A1-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000335879500024},
doi = {10.1021/cg401823k},
url = {https://bib-pubdb1.desy.de/record/168894},
}