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| 001 | 168874 | ||
| 005 | 20250730143958.0 | ||
| 024 | 7 | _ | |a 10.1103/PhysRevB.89.144112 |2 doi |
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| 037 | _ | _ | |a DESY-2014-02701 |
| 082 | _ | _ | |a 530 |
| 100 | 1 | _ | |a Vitova, Tonya |0 P:(DE-H253)PIP1007937 |b 0 |
| 245 | _ | _ | |a X-ray absorption spectroscopy of Ru-doped relaxor ferroelectrics with a perovskite-type structure |
| 260 | _ | _ | |a College Park, Md. |c 2014 |b APS |
| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 336 | 7 | _ | |a article |2 DRIVER |
| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 168874 |2 PUB:(DE-HGF) |
| 336 | 7 | _ | |a ARTICLE |2 BibTeX |
| 520 | _ | _ | |a X-ray absorption near-edge structure and extended x-ray absorption fine structure spectroscopy at the Ru K edge of Ru-doped PbSc0.5Ta0.5O3 (PST-Ru), PbSc0.5Nb0.5O3 (PSN-Ru), and 0.9PbZn1/3Nb2/3O3-0.1PbTiO3 (PZN-0.1PT-Ru) as well as at the Ta L3 edge of PST-Ru and the Nb K edge of PSN-Ru was applied to study the short- and intermediate-range atomic arrangements in perovskite-type (ABO3) relaxor ferroelectrics. The compounds were also analyzed by complementary Raman scattering, visible/near-visible absorption spectroscopy, and synchrotron x-ray single-crystal diffraction. The results show that Ru is octahedrally coordinated in all three relaxor host matrices but the average oxidation state of Ru in PST-Ru and PSN-Ru is ∼4.4, whereas it is ∼3.8 in PZN-0.1PT-Ru. In PbSc0.5B''0.5O3 (B'' = Ta, Nb) Ru substitutes for the B'' cations in the form of isolated point defects, while in PZN-0.1PT-Ru Ru replaces adjacent A and B sites, forming a chainlike structural species of face-sharing elongated octahedra. Chemical 1:1 B-site order as well as dynamic BO6 tilting is observed around both the Ru dopant and the major B'' cation in PST-Ru and PSN-Ru regardless of the fact that according to x-ray diffraction at ambient conditions, the average structure is cubic with weak or no long-range chemical order. Pb cations are off-center displaced from the prototypic cubic A site for all three compounds and in Ru-doped PbSc0.5B''0.5O3 the BO6 tilt angle correlates with the degree of coherent B-Pb distances. |
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| 542 | _ | _ | |i 2014-04-29 |2 Crossref |u http://link.aps.org/licenses/aps-default-license |
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| 700 | 1 | _ | |a Mangold, S. |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Paulmann, Carsten |0 P:(DE-H253)PIP1001761 |b 2 |
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| 773 | 1 | 8 | |a 10.1103/physrevb.89.144112 |b American Physical Society (APS) |d 2014-04-29 |n 14 |p 144112 |3 journal-article |2 Crossref |t Physical Review B |v 89 |y 2014 |x 1098-0121 |
| 773 | _ | _ | |a 10.1103/PhysRevB.89.144112 |0 PERI:(DE-600)2844160-6 |n 14 |p 144112 |t Physical review / B |v 89 |y 2014 |x 1098-0121 |
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