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@ARTICLE{Beye:167779,
author = {Beye, M. and Schreck, S. and Sorgenfrei, F. and Trabant, C.
and Pontius, N. and Schüßler-Langeheine, C. and Wurth, W.
and Föhlisch, A.},
title = {{S}timulated {X}-ray emission for materials science},
journal = {Nature},
volume = {501},
number = {7466},
issn = {1476-4687},
address = {London},
publisher = {Macmillan28177},
reportid = {DESY-2014-02110},
pages = {191 - 194},
year = {2013},
note = {© Macmillan Publishers Limited.},
abstract = {Resonant inelastic X-ray scattering and X-ray emission
spectroscopy can be used to probe the energy and dispersion
of the elementary low-energy excitations that govern
functionality in matter: vibronic, charge, spin and orbital
excitations. A key drawback of resonant inelastic X-ray
scattering has been the need for high photon densities to
compensate for fluorescence yields of less than a per cent
for soft X-rays8. Sample damage from the dominant
non-radiative decays thus limits the materials to which such
techniques can be applied and the spectral resolution that
can be obtained. A means of improving the yield is therefore
highly desirable. Here we demonstrate stimulated X-ray
emission for crystalline silicon at photon densities that
are easily achievable with free-electron lasers. The
stimulated radiative decay of core excited species at the
expense of non-radiative processes reduces sample damage and
permits narrow-bandwidth detection in the directed beam of
stimulated radiation. We deduce how stimulated X-ray
emission can be enhanced by several orders of magnitude to
provide, with high yield and reduced sample damage, a
superior probe for low-energy excitations and their
dispersion in matter. This is the first step to bringing
nonlinear X-ray physics in the condensed phase from theory
to application.},
cin = {DOOR / UNI/EXP},
ddc = {070},
cid = {I:(DE-H253)HAS-User-20120731 /
$I:(DE-H253)UNI_EXP-20120731$},
pnm = {FLASH Beamline PG2 (POF2-54G16) / FLASH Beamline BL2
(POF2-54G16)},
pid = {G:(DE-H253)POF2-PG2-20130405 /
G:(DE-H253)POF2-BL2-20130405},
experiment = {EXP:(DE-H253)F-PG2-20150101 / EXP:(DE-H253)F-BL2-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000324244900034},
pubmed = {pmid:23965622},
doi = {10.1038/nature12449},
url = {https://bib-pubdb1.desy.de/record/167779},
}