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@ARTICLE{Rouze:167681,
      author       = {Rouzée, A. and Johnsson, P. and Rading, L. and
                      Hundertmark, A. and Siu, W. and Huismans, Y. and Düsterer,
                      S. and Redlin, H. and Tavella, F. and Stojanovic, N. and
                      Al-Shemmary, A. and Lépine, F. and Holland, D. M. P. and
                      Schlatholter, T. and Hoekstra, R. and Fukuzawa, H. and Ueda,
                      K. and Vrakking, M. J. J.},
      title        = {{T}owards imaging of ultrafast molecular dynamics using
                      {FEL}s},
      journal      = {Journal of physics / B},
      volume       = {46},
      number       = {16},
      issn         = {1361-6455},
      address      = {Bristol},
      publisher    = {IOP Publ.},
      reportid     = {DESY-2014-02015},
      pages        = {164029},
      year         = {2013},
      note         = {© IOP Publishing Ltd; Post referee fulltext in progress;
                      Embargo 12 months from publication},
      abstract     = {The dissociation dynamics induced by a 100 fs, 400 nm laser
                      pulse in a rotationally cold Br2 sample was characterized by
                      Coulomb explosion imaging (CEI) using a time-delayed extreme
                      ultra-violet (XUV) FEL pulse, obtained from the Free
                      electron LASer in Hamburg (FLASH). The momentum distribution
                      of atomic fragments resulting from the 400 nm-induced
                      dissociation was measured with a velocity map imaging
                      spectrometer and used to monitor the internuclear distance
                      as the molecule dissociated. By employing the simultaneously
                      recorded in-house timing electro-optical sampling data, the
                      time resolution of the final results could be improved to
                      300 fs, compared to the inherent 500 fs time-jitter of the
                      FEL pulse. Before dissociation, the Br2 molecules were
                      transiently 'fixed in space' using laser-induced alignment.
                      In addition, similar alignment techniques were used on CO2
                      molecules to allow the measurement of the photoelectron
                      angular distribution (PAD) directly in the molecular frame
                      (MF). Our results on MFPADs in aligned CO2 molecules,
                      together with our investigation of the dissociation dynamics
                      of the Br2 molecules with CEI, show that information about
                      the evolving molecular structure and electronic geometry can
                      be retrieved from such experiments, therefore paving the way
                      towards the study of complex non-adiabatic dynamics in
                      molecules through XUV time-resolved photoion and
                      photoelectron spectroscopy.},
      cin          = {FS-FL / DOOR / FS-LA},
      ddc          = {530},
      cid          = {I:(DE-H253)FS-FL-20120731 / I:(DE-H253)HAS-User-20120731 /
                      I:(DE-H253)FS-LA-20130416},
      pnm          = {FLASH Beamline BL3 (POF2-54G16)},
      pid          = {G:(DE-H253)POF2-BL3-20130405},
      experiment   = {EXP:(DE-H253)F-BL3-20150101},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000323113100030},
      doi          = {10.1088/0953-4075/46/16/164029},
      url          = {https://bib-pubdb1.desy.de/record/167681},
}