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@ARTICLE{Gorbenko:166883,
author = {Gorbenko, V. and Krasnikov, A. and Mihokova, E. and Nikl,
M. and Zazubovich, S. and Zorenko, Yu.},
title = {{P}hotoluminescence and excited state structure in
${B}i^{3+}$-doped ${L}u_{2}{S}i{O}_{5}$ single crystalline
films},
journal = {Journal of luminescence},
volume = {134},
issn = {1872-7883},
address = {New York, NY [u.a.]},
publisher = {Elsevier},
reportid = {DESY-2014-01681},
pages = {469–476},
year = {2013},
note = {(c) Elsevier B.V.; Post referee fulltext in progress;
Embargo 12 months from publication},
abstract = {Single crystalline films of Lu2SiO5:Bi, prepared by the
liquid phase epitaxy method from the melt-solution based on
Bi2O3 flux, are studied at 4.2–350 K by the time-resolved
spectroscopy methods under excitation in the 2.4–6.2 eV
energy range. An intense dominant ultraviolet (≈3.5 eV)
luminescence of Lu2SiO5:Bi is shown to arise from the
radiative decay of the metastable and radiative minima of
the triplet relaxed excited state (RES) of Bi3+ centers
which are related to the 3P0 and 3P1 levels of a free Bi3+
ion, respectively. At T<50 K, the radiative transitions from
the metastable minima mainly take place. Thermally
stimulated non-radiative transitions between the metastable
and radiative minima of the triplet RES appear at T>50 K in
the temperature evolution of the emission spectrum and decay
kinetics. The excitation bands of the ultraviolet emission,
located at 4.2 eV, 5.03 eV, and 5.95 eV, are assigned to the
1S0→3P1, 1S0→3P2, and 1S0→1P1 transitions of a free
Bi3+ ion, respectively. The phenomenological model is
proposed to describe the excited-state dynamics of Bi3+
centers in Lu2SiO5:Bi. Characteristic parameters of the
triplet RES, in particular the energy separation between the
excited states and the rates of the radiative and
non-radiative transitions from these states, are determined.
Much weaker ≈3.3 eV emission is ascribed to the Bi3+ ions
located in the Lu2 lattice sites. Weak broad ≈2.2 eV and
≈2.3 eV emission bands are assumed to arise from the
Bi3+-related localized excitons.},
cin = {DOOR},
ddc = {530},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {DORIS Beamline I (POF2-54G13) / FS-Proposal: I-20110938 EC
(I-20110938-EC) / CALIPSO - Coordinated Access to
Lightsources to Promote Standards and Optimization (312284)},
pid = {G:(DE-H253)POF2-I-20130405 / G:(DE-H253)I-20110938-EC /
G:(EU-Grant)312284},
experiment = {EXP:(DE-H253)D-I-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000313393300076},
doi = {10.1016/j.jlumin.2012.07.043},
url = {https://bib-pubdb1.desy.de/record/166883},
}