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@ARTICLE{Darul:155271,
author = {Darul, Jolanta and Lathe, Christian and Piszora, Pawel},
title = {${M}n_{3}{O}_{4}$ under {H}igh {P}ressure and
{T}emperature: {T}hermal {S}tability, {P}olymorphism, and
{E}lastic {P}roperties},
journal = {The journal of physical chemistry},
volume = {117},
number = {45},
issn = {1943-300X},
address = {Washington, DC},
publisher = {American Chemical Society},
reportid = {DESY-2013-01390},
pages = {23487-23494},
year = {2013},
note = {© American Chemical Society; Post referee fulltext in
progress; Embargo 12 months from publication},
abstract = {We report results of in situ synchrotron X-ray diffraction
studies of hausmannite up to 7.2 GPa and 1273 K. The Mn3O4
tetragonal spinel is found to transform to a $9.6\%$ denser
polymorph of the CaMn2O4-type structure at 7.2 GPa and 673
K, under milder conditions than those of any transformations
to postspinel phase described so far. Upon heating at high
pressure, the Mn3O4 phase undergoes decomposition and
finally disappears in favor of MnO at temperatures above
1073 K. A fit of the pressure dependence of the volume of
tetragonal phase to the Birch−Murnaghan equation of state
yields the bulk modulus, K0, of 132.6 ± 3.1 GPa if the
first pressure derivative of the bulk modulus is fixed to 4,
and K0, of 102 ± 10 GPa for K0′ refined to 18.1 ± 5.6.
Nonlinear compression behavior is observed for both
crystallographic axes, with the c axis being more
compressible than the a axis. Axial ratios in CaMn2O4-type
Mn3O4 with temperature are also estimated. Surprisingly, the
lattice distortion of the marokite-like phase is not
preserved upon releasing pressure and temperature to ambient
conditions},
cin = {DOOR},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {DORIS Beamline F2.1 (POF2-54G13)},
pid = {G:(DE-H253)POF2-F2.1-20130405},
experiment = {EXP:(DE-H253)D-F2.1-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000327110500006},
doi = {10.1021/jp404852j},
url = {https://bib-pubdb1.desy.de/record/155271},
}